Near-Infrared Fluorescent Probes with Large Stokes Shifts for Sensing Zn(II) Ions in Living Cells

被引：61

作者：

Zhang, Shuwei ^{[1
]}

Adhikari, Rashmi ^{[1
]}

Fang, Mingxi ^{[1
]}

Dorh, Nethaniah ^{[1
]}

Li, Cong ^{[1
]}

Jaishi, Meghnath ^{[2
]}

Zhang, Jingtuo ^{[1
]}

Tiwari, Ashutosh ^{[1
]}

Pati, Ranjit ^{[2
]}

Luo, Fen-Tair ^{[3
]}

Liu, Haiying ^{[1
]}

机构：

[1] Michigan Technol Univ, Dept Chem, Houghton, MI 49931 USA

[2] Michigan Technol Univ, Dept Phys, Houghton, MI 49931 USA

[3] Acad Sinica, Inst Chem, Taipei 11529, Taiwan

来源：

ACS SENSORS | 2016年 / 1卷 / 12期

基金：

美国国家科学基金会; 美国国家卫生研究院;

关键词：

fluorescent probe; near-infrared; Rhodol counterpart; Zn(II) ions; photoinduced electron transfer; ZINC IONS; MOBILE ZINC; ZN2+; SENSORS; RED; CHEMOSENSOR; DESIGN; DYES; PH;

D O I：

10.1021/acssensors.6b00490

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We report two new near-infrared fluorescent probes based on Rhodol counterpart fluorophore platforms functionalized with dipicolylamine Zn(II)-binding groups. The combinations of the pendant amines and fluorophores provide the probes with an effective three-nitrogen-atom and one-oxygen-atom binding motif. The fluorescent probes with large Stokes shifts offer sensitive and selective florescent responses to Zn(II) ions over other metal ions, allowing a reversible monitoring of Zn(II) concentration changes in living cells, and detecting intracellular Zn(II) ions released from intracellular metalloproteins.

引用

页码：1408 / 1415

页数：8

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