Giant Optical Nonlinearity of Graphene in a Strong Magnetic Field

被引:141
作者
Yao, Xianghan [1 ]
Belyanin, Alexey [1 ]
机构
[1] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA
基金
美国国家科学基金会;
关键词
QUANTUM-CASCADE-LASER; MOBILE CARRIERS; GENERATION;
D O I
10.1103/PhysRevLett.108.255503
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We calculate the nonlinear optical response of graphene in strong magnetic and optical fields, using a quantum-mechanical density-matrix formalism. We show that graphene in a magnetic field possesses a giant mid-or far-infrared optical nonlinearity, perhaps the highest among known materials. The high nonlinearity originates from unique electronic properties and selection rules near the Dirac point. As a result, even one monolayer of graphene gives rise to an appreciable nonlinear frequency conversion efficiency for incident infrared radiation.
引用
收藏
页数:5
相关论文
共 21 条
[1]   Optical and magneto-optical far-infrared properties of bilayer graphene [J].
Abergel, D. S. L. ;
Fal'ko, Vladimir I. .
PHYSICAL REVIEW B, 2007, 75 (15)
[2]   Theory of electronic states and transport in carbon nanotubes [J].
Ando, T .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2005, 74 (03) :777-817
[3]   Magnetic oscillation of optical phonon in graphene [J].
Ando, Tsuneya .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2007, 76 (02)
[4]   Terahertz quantum-cascade-laser source based on intracavity difference-frequency generation [J].
Belkin, Mikhail A. ;
Capasso, Federico ;
Belyanin, Alexey ;
Sivco, Deborah L. ;
Cho, Alfred Y. ;
Oakley, Douglas C. ;
Vineis, Christopher J. ;
Turner, George W. .
NATURE PHOTONICS, 2007, 1 (05) :288-292
[5]   THEORY OF OPTICAL MIXING BY MOBILE CARRIERS IN SUPER-LATTICES [J].
BLOSS, WL ;
FRIEDMAN, L .
APPLIED PHYSICS LETTERS, 1982, 41 (11) :1023-1025
[6]   Optimized second-harmonic generation in quantum cascade lasers [J].
Gmachl, C ;
Belyanin, A ;
Sivco, DL ;
Peabody, ML ;
Owschimikow, N ;
Sergent, AM ;
Capasso, F ;
Cho, AY .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 2003, 39 (11) :1345-1355
[7]   Coherent Nonlinear Optical Response of Graphene [J].
Hendry, E. ;
Hale, P. J. ;
Moger, J. ;
Savchenko, A. K. ;
Mikhailov, S. A. .
PHYSICAL REVIEW LETTERS, 2010, 105 (09)
[8]   Infrared spectroscopy of Landau levels of graphene [J].
Jiang, Z. ;
Henriksen, E. A. ;
Tung, L. C. ;
Wang, Y. -J. ;
Schwartz, M. E. ;
Han, M. Y. ;
Kim, P. ;
Stormer, H. L. .
PHYSICAL REVIEW LETTERS, 2007, 98 (19)
[9]   Quantum spin hall insulator state in HgTe quantum wells [J].
Koenig, Markus ;
Wiedmann, Steffen ;
Bruene, Christoph ;
Roth, Andreas ;
Buhmann, Hartmut ;
Molenkamp, Laurens W. ;
Qi, Xiao-Liang ;
Zhang, Shou-Cheng .
SCIENCE, 2007, 318 (5851) :766-770
[10]   Nonlinear cyclotron resonance of a massless quasiparticle in graphene [J].
Mikhailov, S. A. .
PHYSICAL REVIEW B, 2009, 79 (24)