Characteristics and assessment of phthalate esters in urban dusts in Guangzhou city, China

被引:54
作者
Lan, Qing [1 ]
Cui, Kunyan [2 ]
Zeng, Feng [1 ]
Zhu, Fang [1 ]
Liu, Hong [1 ]
Chen, Hongli [1 ]
Ma, Yongqing [1 ]
Wen, Jiaxin [1 ]
Luan, Tiangang [3 ]
Sun, Guoquan [4 ]
Zeng, Zunxiang [1 ]
机构
[1] Sun Yat Sen Univ, Sch Chem & Chem Engn, Guangzhou 510275, Guangdong, Peoples R China
[2] Sun Yat Sen Univ, Instrumental Anal & Res Ctr, Guangzhou 510275, Guangdong, Peoples R China
[3] Sun Yat Sen Univ, Sch Life Sci, MOE Key Lab Aquat Prod Safety, State Key Lab Biocontrol, Guangzhou 510275, Guangdong, Peoples R China
[4] E China Inst Technol, Dept Appl Chem, Fuzhou 344000, Jiangxi, Peoples R China
基金
中国国家自然科学基金;
关键词
Phthalate esters; Urban dust; Guangzhou; Human exposure; POLYBROMINATED DIPHENYL ETHERS; AROMATIC-HYDROCARBONS PAHS; DIBENZO-P-DIOXINS; INDOOR DUST; SUBTROPICAL CITY; SETTLED DUST; ACID ESTERS; SOUTH CHINA; GAS-PHASE; EXPOSURE;
D O I
10.1007/s10661-011-2312-3
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Phthalate esters (PAEs) were examined in indoor and outdoor dust samples from the subtropical city of Guangzhou, China. The a(16)PAEs concentrations ranged from 121 to 3,223 mu g g(-1) dust, with the median concentration of 840 mu g g(-1) dust. Significantly higher concentrations of PAEs in dust samples were found in offices where electrical and electronic devices, carpet pads, and office furniture were widely used. Of the 16 PAEs, diisobutyl phthalate (DiBP), di-n-butyl phthalate (DnBP), and di(2-ethylhexyl) phthalate (DEHP) dominated the PAEs in indoor and outdoor dust samples, and accounted for > 96.8% and > 93.1% of the a(16)PAEs concentrations, respectively. The median daily inhalation exposure of a(16)PAEs were 3.53 and 0.247 mu g kg(-1) body weight day(-1), and at the 95(th) percentile were 7.62 and 0.530 mu g kg(-1) body weight day(-1), up on the measured concentrations and estimated dust ingestion rates, respectively, for toddles and adults. The ubiquitous distribution of PAEs as noted in this study suggests the need for detailed assessment of PAEs concentrations using more sites and to further investigate the factors influencing PAEs exposure in China.
引用
收藏
页码:4921 / 4929
页数:9
相关论文
共 47 条
[1]   Phthalates in house dust [J].
Abb, M. ;
Heinrich, T. ;
Sorkau, E. ;
Lorenz, W. .
ENVIRONMENT INTERNATIONAL, 2009, 35 (06) :965-970
[2]   Hexabromocyclododecanes in indoor dust from Canada, the United Kingdom, and-the United States [J].
Abdallah, Mohamed Abou-Elwafa ;
Harrad, Stuart ;
Ibarra, Catalina ;
Diamond, Miriam ;
Melymuk, Lisa ;
Robson, Matthew ;
Covaci, Adrian .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2008, 42 (02) :459-464
[3]   DEHP metabolites in urine of children and DEHP in house dust [J].
Becker, K ;
Seiwert, M ;
Angerer, J ;
Heger, W ;
Koch, HM ;
Nagorka, R ;
Rosskamp, E ;
Schlüter, C ;
Seifert, B ;
Ullrich, D .
INTERNATIONAL JOURNAL OF HYGIENE AND ENVIRONMENTAL HEALTH, 2004, 207 (05) :409-417
[4]   Phthalates in indoor dust and their association with building characteristics [J].
Bornehag, CG ;
Lundgren, B ;
Weschler, CJ ;
Sigsgaard, T ;
Hagerhed-Engman, L ;
Sundell, J .
ENVIRONMENTAL HEALTH PERSPECTIVES, 2005, 113 (10) :1399-1404
[5]   The status of soil contamination by semivolatile organic chemicals (SVOCs) in China: A review [J].
Cai, Quan-Ying ;
Mo, Ce-Hui ;
Wu, Qi-Tang ;
Katsoyiannis, Athanasios ;
Zeng, Qiao-Yun .
SCIENCE OF THE TOTAL ENVIRONMENT, 2008, 389 (2-3) :209-224
[6]   In- and outdoor sources of polybrominated diphenyl ethers and their human inhalation exposure in Guangzhou, China [J].
Chen, Laiguo ;
Mai, Bixian ;
Xu, Zhencheng ;
Peng, Xiaochun ;
Han, Jinglel ;
Ran, Yong ;
Sheng, Guoying ;
Fu, Jiamo .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (01) :78-86
[7]   Seasonal variation on size distribution and concentration of PAHs in Guangzhou city, China [J].
Duan, Jingchun ;
Bi, Xinhui ;
Tan, Jlhua ;
Sheng, Guoying ;
Fu, Jiamo .
CHEMOSPHERE, 2007, 67 (03) :614-622
[8]   Occurrence of phthalates and musk fragrances in indoor air and dust from apartments and kindergartens in Berlin (Germany) [J].
Fromme, H ;
Lahrz, T ;
Piloty, M ;
Gebhart, H ;
Oddoy, A ;
Rüden, H .
INDOOR AIR, 2004, 14 (03) :188-195
[9]   Elucidation of the toxic mechanism of the plasticizers, phthalic acid esters, putative endocrine disrupters: Effects of dietary di(2-ethylhexyl)phthalate on the metabolism of tryptophan to niacin in rats [J].
Fukuwatari, T ;
Suzuki, Y ;
Sugimoto, E ;
Shibata, K .
BIOSCIENCE BIOTECHNOLOGY AND BIOCHEMISTRY, 2002, 66 (04) :705-710
[10]   Environmental pathways of exposure to DDT for children living in a malarious area of Chiapas, Mexico [J].
Herrera-Portugal, C ;
Ochoa, H ;
Franco-Sánchez, G ;
Yáñez, L ;
Díaz-Barriga, F .
ENVIRONMENTAL RESEARCH, 2005, 99 (02) :158-163