Effect of gas temperature on partial oxidation of methane in plasma reforming

被引：27

作者：

Jo, Sungkwon ^{[1
]}

Lee, Dae Hoon ^{[1
]}

Song, Young-Hoon ^{[1
]}

机构：

[1] Korea Inst Machinery & Mat, Plasma Lab, Taejon 305343, South Korea

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2013年 / 38卷 / 31期

关键词：

Plasma reforming; Methane; Synthesis gas; Reaction pathway; NONTHERMAL PLASMA; CONVERSION; REACTOR;

D O I：

10.1016/j.ijhydene.2013.08.049

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Plasma-reforming process has been widely studied for over a decade, with a focus on diverse fuels and plasma parameters for finding the optimum conditions. This study evaluates the effect of thermal activation on the chemistry and energy efficiency of the methane-reforming process. Based on the empirical evaluation, a correlation was found among the methane conversion rate, reaction composition, reactant temperature, and plasma power. Moreover, the plasma chemistry did not change with the reactant temperature within the temperature range evaluated. In addition, it was found that the ratio of the plasma power to the heating input power was an important parameter for enhancing the efficiency of the partial oxidation of methane. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.

引用

页码：13643 / 13648

页数：6

共 13 条

[1] Review of plasma catalysis on hydrocarbon reforming for hydrogen production-Interaction, integration, and prospects [J].

Chen, Hsin Liang ;

Lee, How Ming ;

Chen, Shiaw Huei ;

Chao, Yu ;

Chang, Moo Been .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2008, 85 (1-2) :1-9

[2]

Fridman A., 2008, PLASMA CHEM

[3] Plasma-assisted partial oxidation of methane at low temperatures: numerical analysis of gas-phase chemical mechanism [J].

Goujard, Valentin ;

Nozaki, Tomohiro ;

Yuzawa, Shuhei ;

Agiral, Anil ;

Okazaki, Ken .

JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2011, 44 (27)

[4] Combustion-assisted plasma in fuel conversion [J].

Gutsol, A. ;

Rabinovich, A. ;

Fridman, A. .

JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2011, 44 (27)

[5] Optimization scheme of a rotating gliding arc reactor for partial oxidation of methane [J].

Lee, D. H. ;

Kim, K. -T. ;

Cha, M. S. ;

Song, Y. -H. .

PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2007, 31 :3343-3351

[6] Mapping Plasma Chemistry in Hydrocarbon Fuel Processing Processes [J].

Lee, Dae Hoon ;

Kim, Kwan-Tae ;

Song, Young-Hoon ;

Kang, Woo Suk ;

Jo, Sungkwon .

PLASMA CHEMISTRY AND PLASMA PROCESSING, 2013, 33 (01) :249-269

[7] Plasma-controlled chemistry in plasma reforming of methane [J].

Lee, Dae Hoon ;

Kim, Kuian-Tae ;

Cha, Min Suk ;

Song, Young-Hoon .

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2010, 35 (20) :10967-10976

[8] Partial oxidation of methane using a microscale non-equilibrium plasma reactor [J].

Nozaki, T ;

Hattori, A ;

Okazaki, K .

CATALYSIS TODAY, 2004, 98 (04) :607-616

[9] Chemical reaction kinetics and reactor modeling of NOx removal in a pulsed streamer corona discharge reactor [J].

Sathiamoorthy, G ;

Kalyana, S ;

Finney, WC ;

Clark, RJ ;

Locke, BR .

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1999, 38 (05) :1844-1855

[10] Plasma assisted ignition and combustion [J].

Starikovskaia, S. M. .

JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2006, 39 (16) :R265-R299

← 1 2 →