Collective resonances in χ(3): A QED study

被引：6

作者：

Dorfman, Konstantin E. ^{[1
]}

Mukamel, Shaul ^{[1
]}

机构：

[1] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA

来源：

PHYSICAL REVIEW A | 2013年 / 87卷 / 06期

基金：

美国国家科学基金会;

关键词：

STOKES-RAMAN SCATTERING; LASER; SPECTROSCOPY; DYNAMICS; PHASE;

D O I：

10.1103/PhysRevA.87.063831

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We calculate the third-order susceptibility chi((3)) of a pair of two-level atoms that interact via the exchange of photons. QED corrections to second order in coupling to vacuum field modes yield collective two-photon absorption resonances, which can be observed in transmission spectroscopy of shaped broadband pulses. While some collective effects can be obtained by introducing an effective interatomic coupling using a quantum master equation, the predicted signals contain distinct features that are missed by that level of theory and require a full diagrammatic QED treatment.

引用

页数：13

共 40 条

[21] Imaging the thermodynamic state of lipid membranes with multiplex CARS microscopy [J].

Müller, M ;

Schins, JM .

JOURNAL OF PHYSICAL CHEMISTRY B, 2002, 106 (14) :3715-3723

[22]

Nielsen M. A, 2002, QUANTUM COMPUTATION

[23] Ultrafast spectroscopy of QUANTUM MATERIALS [J].

Orenstein, Joseph .

PHYSICS TODAY, 2012, 65 (09) :44-50

[24] Optimizing the laser-pulse configuration for coherent Raman spectroscopy [J].

Pestov, Dmitry ;

Murawski, Robert K. ;

Ariunbold, Gombojav O. ;

Wang, Xi ;

Zhi, Miaochan ;

Sokolov, Alexei V. ;

Sautenkov, Vladimir A. ;

Rostovtsev, Yuri V. ;

Dogariu, Arthur ;

Huang, Yu ;

Scully, Marlan O. .

SCIENCE, 2007, 316 (5822) :265-268

[25] MAXWELLS EQUATIONS AND THE MULTIPOLAR HAMILTONIAN [J].

POWER, EA ;

THIRUNAMACHANDRAN, T .

PHYSICAL REVIEW A, 1982, 26 (03) :1800-1801

[26] THE MULTIPOLAR HAMILTONIAN IN RADIATION THEORY [J].

POWER, EA ;

THIRUNAMACHANDRAN, T .

PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1980, 372 (1749) :265-273

[27] Single-Photon Spectroscopy of a Single Molecule [J].

Rezus, Y. L. A. ;

Walt, S. G. ;

Lettow, R. ;

Renn, A. ;

Zumofen, G. ;

Goetzinger, S. ;

Sandoghdar, V. .

PHYSICAL REVIEW LETTERS, 2012, 108 (09)

[28] Collective two-particle resonances induced by photon entanglement [J].

Richter, Marten ;

Mukamel, Shaul .

PHYSICAL REVIEW A, 2011, 83 (06)

[29] Single-beam coherent anti-Stokes Raman scattering (CARS) spectroscopy of gas-phase CO2 via phase and polarization shaping of a broadband continuum [J].

Roy, Sukesh ;

Wrzesinski, Paul J. ;

Pestov, Dmitry ;

Dantus, Marcos ;

Gord, James R. .

JOURNAL OF RAMAN SPECTROSCOPY, 2010, 41 (10) :1194-1199

[30]

Salam A., 2010, Molecular Quantum Electrodynamics, DOI DOI 10.1002/9780470535462

← 1 2 3 4 →