Collective resonances in χ(3): A QED study

被引：5

作者：

Dorfman, Konstantin E. ^{[1
]}

Mukamel, Shaul ^{[1
]}

机构：

[1] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA

来源：

PHYSICAL REVIEW A | 2013年 / 87卷 / 06期

基金：

美国国家科学基金会;

关键词：

STOKES-RAMAN SCATTERING; LASER; SPECTROSCOPY; DYNAMICS; PHASE;

D O I：

10.1103/PhysRevA.87.063831

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We calculate the third-order susceptibility chi((3)) of a pair of two-level atoms that interact via the exchange of photons. QED corrections to second order in coupling to vacuum field modes yield collective two-photon absorption resonances, which can be observed in transmission spectroscopy of shaped broadband pulses. While some collective effects can be obtained by introducing an effective interatomic coupling using a quantum master equation, the predicted signals contain distinct features that are missed by that level of theory and require a full diagrammatic QED treatment.

引用

页数：13

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