Collective resonances in χ(3): A QED study

被引：5
作者：
Dorfman, Konstantin E. [1 ]
Mukamel, Shaul [1 ]
机构：
[1] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA
来源：
PHYSICAL REVIEW A | 2013年 / 87卷 / 06期
基金：
美国国家科学基金会;
关键词：
STOKES-RAMAN SCATTERING; LASER; SPECTROSCOPY; DYNAMICS; PHASE;
D O I：
10.1103/PhysRevA.87.063831
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
We calculate the third-order susceptibility chi((3)) of a pair of two-level atoms that interact via the exchange of photons. QED corrections to second order in coupling to vacuum field modes yield collective two-photon absorption resonances, which can be observed in transmission spectroscopy of shaped broadband pulses. While some collective effects can be obtained by introducing an effective interatomic coupling using a quantum master equation, the predicted signals contain distinct features that are missed by that level of theory and require a full diagrammatic QED treatment.
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页数：13
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