Potential Source Regions Contributing to Seasonal Variations of Black Carbon Aerosols over Anantapur in Southeast India

被引:50
作者
Reddy, B. Suresh Kumar [1 ,6 ]
Kumar, K. Raghavendra [1 ]
Balakrishnaiah, G. [1 ,5 ]
Gopal, K. Rama [1 ]
Reddy, R. R. [1 ]
Reddy, L. S. S. [1 ]
Ahammed, Y. Nazeer [2 ]
Narasimhulu, K. [3 ]
Moorthy, K. Krishna [4 ]
Babu, S. Suresh [4 ]
机构
[1] Sri Krishnadevaraya Univ, Dept Phys, Aerosol & Atmospher Res Lab, Anantapur 515055, Andhra Pradesh, India
[2] Yogi Vemana Univ, Dept Phys, Kadapa 516003, Andhra Pradesh, India
[3] Govt First Grade Coll, Dept Phys, Bellary 583101, Karnataka, India
[4] Vikram Sarabhai Space Ctr, Space Phys Lab, Trivandrum 695022, Kerala, India
[5] Natl Chiao Tung Univ, Inst Environm Engn, Hsinchu 300, Taiwan
[6] Hokkaido Univ, Inst Low Temp Sci, Sapporo, Hokkaido 0600819, Japan
关键词
BC aerosol; Potential sources regions; AOD; Angstrom exponent; PM2.5; LONG-RANGE TRANSPORT; 7-WAVELENGTH AETHALOMETER; ABSORPTION-MEASUREMENTS; TEMPORAL VARIATIONS; MASS CONCENTRATION; URBAN-ENVIRONMENT; SIZE DISTRIBUTION; LIGHT-ABSORPTION; PM2.5; PARTICLES;
D O I
10.4209/aaqr.2011.10.0159
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Continuous measurements of black carbon (BC) mass concentration performed at Anantapur [14.62 degrees N, 77.65 degrees E, 331 m asl], a suburban location in southeast India, using an Aethalometer from January to December, 2010, are analyzed and discussed here. The annual mean BC mass concentration ([BC]) was 3.03 +/- 0.27 mu g/m(3) for the above study period. The sharp morning (fumigation) peak occurs between 07:00 and 08:00 h almost an hour after the local sunrise while a broad evening (nocturnal) peak is at similar to 21:00 h with a minimum in noon hours (14:00-16:00 h). The seasonal mean values of [BC] are 5.05 +/- 0.51 mu g/m(3) in the winter, 3.77 +/- 1.23, 1.55 +/- 0.51, and 2.33 +/- 0.82 mu g/m(3) in the summer, monsoon and postmonsoon seasons, respectively. High BC values tend to occur when the wind is directed from the 180-225 degrees sector, which may be well defined by the geographical location of the observation site. During the winter, the trajectory air mass pathways originated through north or central India with significant advection of continental aerosols arriving before the measurement region, results in an enhanced [BC]. Whereas in the monsoon season, the pristine marine air mass from the oceanic environment led to decrease in the concentration of BC. Comparison of monthly mean variations in AOD at 500 nm and black carbon aerosols is observed to be positive with poor correlation coefficient of 0.42. The ratio of BC/PM2.5 varied from 1.3% to 7.2% with a mean value of 4.6% at Anantapur during the observation period and this ratio decreased with decreasing Angstrom exponent (alpha).
引用
收藏
页码:344 / 358
页数:15
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