Multiple-photon excitation of nitrogen vacancy centers in diamond

被引：18

作者：

Ji, Peng ^{[1
]}

Balili, R. ^{[2
]}

Beaumariage, J. ^{[1
]}

Mukherjee, S. ^{[1
]}

Snoke, D. ^{[1
]}

Dutt, M. V. Gurudev ^{[1
]}

机构：

[1] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA

[2] Calvin Coll, Dept Phys & Astron, Grand Rapids, MI 49546 USA

来源：

PHYSICAL REVIEW B | 2018年 / 97卷 / 13期

关键词：

NANODIAMONDS; FLUORESCENCE;

D O I：

10.1103/PhysRevB.97.134112

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

We report the observation of multiphoton photoluminescence excitation (PLE) below the resonant energies of nitrogen vacancy (NV) centers in diamond. The quadratic and cubic dependence of the integrated fluorescence intensity as a function of excitation power indicates a two-photon excitation pathway for the NV- charge state and a three-photon process involved for the neutral NV0 charge state, respectively. Comparing the total multiphoton energy with its single-photon equivalent, the PLE spectra follows the absorption spectrum of single photon excitation. We also observed that the efficiency of photoluminescence for different charge states, as well as the decay time constant, was dependent on the excitation wavelength and power.

引用

页数：6

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