0D/2D Fe2O3 quantum dots/g-C3N4 for enhanced visible-light-driven photocatalysis

被引:60
作者
Hao, Quanguo [1 ]
Mo, Zhao [1 ]
Chen, Zhigang [1 ]
She, Xiaojie [1 ]
Xu, Yuanguo [1 ]
Song, Yanhua [2 ]
Ji, Haiyan [1 ]
Wu, Xiangyang [1 ]
Yuan, Shouqi [1 ]
Xu, Hui [1 ]
Li, Huaming [1 ]
机构
[1] Jiangsu Univ, Inst Energy Res, Sch Environm & Safety Engn, Zhenjiang 212013, Peoples R China
[2] Jiangsu Univ Sci & Technol, Sch Environm & Chem Engn, Zhenjiang 212003, Peoples R China
关键词
Fe2O3; QDs; 2D-C3N4; Photocatalytic degradation; High stability; GRAPHITIC CARBON NITRIDE; 2D G-C3N4 NANOSHEETS; IN-SITU SYNTHESIS; HYDROGEN EVOLUTION; FACILE SYNTHESIS; HIGH-PERFORMANCE; H-2; EVOLUTION; DOPED G-C3N4; WATER; NANOPARTICLES;
D O I
10.1016/j.colsurfa.2018.01.023
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
0D/2D photocatalysts have aroused concern due to the high charge mobility. Herein, a 0D/2D structure is formed by employing a facile method to disperse Fe2O3 Quantum-Dots (QDs) on 2D-C3N4 without aggregation at a relatively low temperature of 200 degrees C. The ultrathin monolayer 2D structure, highly dispersed Fe2O3 QDs, the strong coupling as well as quantum-sized confinement effect between them lead to superior visible-light-driven photocurrent performance and photocatalytic activity. Particularly, the 0.5% Fe2O3 QDs/2D-C3N4 composite exhibits the highest photocatalytic activity under visible light. More importantly, the 0D/2D photocatalysts show superior durability with little photocatalytic activity decline in the circular reaction for the photocatalytic degradation of organic pollution. Therefore, this work supplies a new opportunity to construct multifunctional 0D/2D photocatalysts for degradation of pollutants in water.
引用
收藏
页码:188 / 194
页数:7
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