Low cost measurements of nitrogen and sulphur dry deposition velocities at a semi-alpine site: Gradient measurements and a comparison with deposition model estimates

被引:12
作者
Hole, Lars R. [1 ]
Brunner, Sibyl H. [1 ,4 ]
Hanssen, Jan Erik [2 ]
Zhang, Leiming [3 ]
机构
[1] Norwegian Inst Air Res, Dept Atmosphere & Climate, Polar Environm Ctr, N-9296 Tromso, Norway
[2] Norwegian Inst Air Res, Dept Environm Chem, N-2027 Kjeller, Norway
[3] Environm Canada, Sci & Technol Branch, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
[4] Swiss Fed Inst Technol, Zurich, Switzerland
基金
奥地利科学基金会;
关键词
dry deposition; gradient measurement; model comparison; nitrogen; sulphur;
D O I
10.1016/j.envpol.2007.06.061
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The conditional time averaged gradient method was used to measure air-surface exchange of nitrogen and sulphur compounds at a semi-alpine site ill Southern Norway. Dry deposition velocities were then obtained from the bi-weekly concentration gradient measurements. Annual deposition velocities were found to be 1.4, 11.8 and 4.0 mm s(-1) for NH3, HNO3 and SO2, respectively, if all data were included, and to be 10.8. 11.8 and 13.0 mm s(-1), respectively, if only Positive values were included. Measured deposition velocities were compared 10 two sets of values estimated from a big-leaf dry deposition module applying to two different land types (short grass and forbs, and tundra), driven by measured micrormeteorological parameters. The deposition module gives reasonable values for this site throughout the year, but does not reproduce the large variability Lis shown in the measured data. No apparent seasonal variations were found from either measurements or Module estimates due to the very low productivity of the studied area. (C) 2007 Elsevier Ltd. All rights reserved.
引用
收藏
页码:473 / 481
页数:9
相关论文
共 26 条
[1]   Atmospheric nitrogen compounds II: emissions, transport, transformation, deposition and assessment [J].
Aneja, VP ;
Roelle, PA ;
Murray, GC ;
Southerland, J ;
Erisman, JW ;
Fowler, D ;
Asman, WAH ;
Patni, N .
ATMOSPHERIC ENVIRONMENT, 2001, 35 (11) :1903-1911
[2]  
BRUNNER S, 2007, ANAL DRY DEPOSITION
[3]  
Erisman J. W., 2001, WATER AIR SOIL POLL, V1, P17, DOI [10.1023/A:1013105727252, DOI 10.1023/A:1013105727252]
[4]   CONTINUOUS MEASUREMENTS OF SURFACE EXCHANGE OF SO(2) AND NH(3) - IMPLICATIONS FOR THEIR POSSIBLE INTERACTION IN THE DEPOSITION PROCESS [J].
ERISMAN, JW ;
WYERS, GP .
ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS, 1993, 27 (13) :1937-1949
[5]   Deposition monitoring networks: what monitoring is required to give reasonable estimates of ammonia/ammonium? [J].
Erisman, JW ;
Hensen, A ;
Mosquera, J ;
Sutton, M ;
Fowler, D .
ENVIRONMENTAL POLLUTION, 2005, 135 (03) :419-431
[6]   Monitoring and modelling of biosphere/atmosphere exchange of gases and aerosols in Europe [J].
Erisman, JW ;
Vermeulen, A ;
Hensen, A ;
Flechard, C ;
Dämmgen, U ;
Fowler, D ;
Sutton, M ;
Grünhage, L ;
Tuovinen, JP .
ENVIRONMENTAL POLLUTION, 2005, 133 (03) :403-413
[7]  
FAMULARI D, DEV LOW COST S UNPUB
[8]   Evaluation of SO2 dry deposition over short vegetation in Portugal [J].
Feliciano, MS ;
Pio, CA ;
Vermeulen, AT .
ATMOSPHERIC ENVIRONMENT, 2001, 35 (21) :3633-3643
[9]   Long term measurements of the land-atmosphere exchange of ammonia over moorland [J].
Fowler, D ;
Flechard, CR ;
Sutton, MA ;
Storeton-West, RL .
ATMOSPHERIC ENVIRONMENT, 1998, 32 (03) :453-459
[10]   Advances in micrometeorological methods for the measurement and interpretation of gas and particle nitrogen fluxes [J].
Fowler, D ;
Coyle, M ;
Flechard, C ;
Hargreaves, K ;
Nemitz, E ;
Storeton-West, R ;
Sutton, M ;
Erisman, JW .
PLANT AND SOIL, 2001, 228 (01) :117-129