Deep Inner-Shell Multiphoton Ionization by Intense X-Ray Free-Electron Laser Pulses

被引：127

作者：

Fukuzawa, H. ^{[1
,2
]}

Son, S. -K. ^{[3
]}

Motomura, K. ^{[1
]}

Mondal, S. ^{[1
]}

Nagaya, K. ^{[2
,4
]}

Wada, S. ^{[2
,5
]}

Liu, X. -J. ^{[6
]}

Feifel, R. ^{[7
]}

Tachibana, T. ^{[1
]}

Ito, Y. ^{[1
]}

Kimura, M. ^{[1
]}

Sakai, T. ^{[4
]}

Matsunami, K. ^{[4
]}

Hayashita, H. ^{[5
]}

Kajikawa, J. ^{[5
]}

Johnsson, P. ^{[8
]}

Siano, M. ^{[9
]}

Kukk, E. ^{[10
]}

Rudek, B. ^{[11
,12
]}

Erk, B. ^{[11
,12
]}

Foucar, L. ^{[11
,13
]}

Robert, E. ^{[6
]}

Miron, C. ^{[6
]}

Tono, K. ^{[14
]}

Inubushi, Y. ^{[2
]}

Hatsui, T. ^{[2
]}

Yabashi, M. ^{[2
]}

Yao, M. ^{[4
]}

Santra, R. ^{[3
,15
]}

Ueda, K. ^{[1
,2
]}

机构：

[1] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan

[2] RIKEN SPring 8 Ctr, Sayo, Hyogo 6795148, Japan

[3] Ctr Free Elect Laser Sci CFEL, D-22607 Hamburg, Germany

[4] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan

[5] Hiroshima Univ, Dept Phys Sci, Higashihiroshima 7398526, Japan

[6] Synchrotron SOLEIL Orme Merisiers, FR-91192 Gif Sur Yvette, France

[7] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden

[8] Lund Univ, Dept Phys, S-22100 Lund, Sweden

[9] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2AZ, England

[10] Univ Turku, Dept Phys & Astron, Turku 20014, Finland

[11] Max Planck Adv Study Grp CFEL, D-22607 Hamburg, Germany

[12] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany

[13] Max Planck Inst Med Res, D-69120 Heidelberg, Germany

[14] Japan Synchrotron Radiat Res Inst JASRI, Sayo, Hyogo 6795198, Japan

[15] Univ Hamburg, Dept Phys, D-20355 Hamburg, Germany

来源：

PHYSICAL REVIEW LETTERS | 2013年 / 110卷 / 17期

基金：

瑞典研究理事会; 日本学术振兴会;

关键词：

EXTREME-ULTRAVIOLET; ATOMS; OPERATION; REGION;

D O I：

10.1103/PhysRevLett.110.173005

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We have investigated multiphoton multiple ionization dynamics of xenon atoms using a new x-ray free-electron laser facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that Xen+ with n up to 26 is produced at a photon energy of 5.5 keV. The observed high charge states (n >= 24) are produced via five-photon absorption, evidencing the occurrence of multiphoton absorption involving deep inner shells. A newly developed theoretical model, which shows good agreement with the experiment, elucidates the complex pathways of sequential electronic decay cascades accessible in heavy atoms. The present study of heavy-atom ionization dynamics in high-intensity hard-x-ray pulses makes a step forward towards molecular structure determination with x-ray free-electron lasers. DOI: 10.1103/PhysRevLett.110.173005

引用

页数：5

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