Double Core-Hole Creation by Sequential Attosecond Photoionization

被引：50

作者：

Tamasaku, Kenji ^{[1
]}

Nagasono, Mitsuru ^{[1
]}

Iwayama, Hiroshi ^{[2
]}

Shigemasa, Eiji ^{[2
]}

Inubushi, Yuichi ^{[1
]}

Tanaka, Takashi ^{[1
]}

Tono, Kensuke ^{[3
]}

Togashi, Tadashi ^{[3
]}

Sato, Takahiro ^{[1
]}

Katayama, Tetsuo ^{[3
]}

Kameshima, Takashi ^{[3
]}

Hatsui, Takaki ^{[1
]}

Yabashi, Makina ^{[1
]}

Ishikawa, Tetsuya ^{[1
]}

机构：

[1] RIKEN SPring 8 Ctr, Mikazuki, Hyogo 6795148, Japan

[2] IMS, UVSOR Facil, Nagoya, Aichi 4448585, Japan

[3] JASRI, Mikazuki, Hyogo 6795148, Japan

来源：

PHYSICAL REVIEW LETTERS | 2013年 / 111卷 / 04期

关键词：

FREE-ELECTRON LASER; ANOMALOUS DIFFRACTION; FEMTOSECOND LASER; PULSES; ATOMS;

D O I：

10.1103/PhysRevLett.111.043001

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

X-ray fluorescence spectroscopy demonstrates that a single core-hole krypton with a 170-as lifetime can be photoionized again to a double core-hole state by an intense x-ray pulse. The observation indicates that unconventional interaction between intense x rays and atoms is no more negligible in applications with x-ray free-electron lasers. Quantitative analysis of the double core-hole creation including effects of a pulsed and spiky temporal structure enables estimation of the x-ray pulse duration in the sub-10-fs range.

引用

页数：5

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