Decorrelation of the static and dynamic length scales in hard-sphere glass formers

被引:66
作者
Charbonneau, Patrick [1 ,2 ]
Tarjus, Gilles [3 ]
机构
[1] Duke Univ, Dept Chem, Durham, NC 27708 USA
[2] Duke Univ, Dept Phys, Durham, NC 27708 USA
[3] Univ Paris 06, LPTMC, CNRS UMR 7600, F-75252 Paris 05, France
来源
PHYSICAL REVIEW E | 2013年 / 87卷 / 04期
关键词
GROWING LENGTH; ORDER; LIQUIDS;
D O I
10.1103/PhysRevE.87.042305
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We show that, in the equilibrium phase of glass-forming hard-sphere fluids in three dimensions, the static length scales tentatively associated with the dynamical slowdown and the dynamical length characterizing spatial heterogeneities in the dynamics unambiguously decorrelate. The former grow at a much slower rate than the latter when density increases. This observation is valid for the dynamical range that is accessible to computer simulations, which roughly corresponds to that accessible in colloidal experiments. We also find that, in this same range, no one-to-one correspondence between relaxation time and point-to-set correlation length exists. These results point to the coexistence of several relaxation mechanisms in the dynamically accessible regime of three-dimensional hard-sphere glass formers. DOI: 10.1103/PhysRevE.87.042305
引用
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页数:8
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