Ignition behavior of single coal particle in a fluidized bed under O2/CO2 and O2/N2 atmospheres: A combination of visual image and particle temperature

被引:61
作者
Bu, Changsheng [1 ]
Liu, Daoyin [1 ]
Chen, Xiaoping [1 ]
Pallares, David [2 ]
Gomez-Barea, Alberto [3 ]
机构
[1] Southeast Univ, Sch Energy & Environm, Minist Educ, Key Lab Energy Thermal Convers & Control, Nanjing 210096, Jiangsu, Peoples R China
[2] Chalmers, Environm & Energy Dept, S-41296 Gothenburg, Sweden
[3] Univ Seville, Chem & Environm Engn Dept, Seville 41092, Spain
基金
中国国家自然科学基金;
关键词
Oxyfuel; O-2/CO2; atmosphere; Fluidized bed; Devolatilization; Ignition; OXY-FUEL COMBUSTION; HYDROGEN-PRODUCTION SYSTEMS; PULVERIZED COAL; CO2; CAPTURE; DIFFERENT RANKS; CHAR PARTICLES; DEVOLATILIZATION; GASIFICATION; PYROLYSIS; ELECTRICITY;
D O I
10.1016/j.apenergy.2013.10.040
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Single coal particle ignition behavior was studied in a two-dimensional (200 mm x 20 mm x 400 mm) fluidized bed under O-2/N-2 and O-2/CO2 atmosphere with O-2 volume concentration in the range of 0-40%, by a combination of visual observation of the volatile flame and measurement of the particle center temperature. A piece of transparent quartz glass was used as the front wall of the fluidized bed to allow visual observation. The investigated fuel particles were spherical sub-bituminous coal particles with diameter in a range of 6-13 mm, which were artificially carved from selected original coal particles. The volatile combustion flame was recorded by a color video camera to analyze its ignition time delay and extinction behavior. The temperature in the particle center was measured by a very thin thermocouple to follow the particle heating process. Results indicate that under O-2/CO2 atmosphere the ignition delay time is much longer than in O-2/N-2 atmosphere. The devolatilization process is controlled by internal and external heat transfer but it is almost unaffected by atmosphere at the same O-2 concentration. The effect of volatile combustion on heating and extinction delay time can be neglected for larger coal particles. (C) 2013 Elsevier Ltd. All rights reserved.
引用
收藏
页码:301 / 308
页数:8
相关论文
共 39 条
[31]   Particle imaging of ignition and devolatilization of pulverized coal during oxy-fuel combustion [J].
Shaddix, Christopher R. ;
Molina, Alejandro .
PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2009, 32 :2091-2098
[32]   COAL PYROLYSIS - EXPERIMENTS, KINETIC RATES AND MECHANISMS [J].
SOLOMON, PR ;
SERIO, MA ;
SUUBERG, EM .
PROGRESS IN ENERGY AND COMBUSTION SCIENCE, 1992, 18 (02) :133-220
[33]   Effects of steam on the sulfation of limestone and NOx formation in an air- and oxy-fired pilot-scale circulating fluidized bed combustor [J].
Stewart, Michael C. ;
Symonds, Robert T. ;
Manovic, Vasilije ;
Macchi, Arturo ;
Anthony, Edward J. .
FUEL, 2012, 92 (01) :107-115
[34]   Alstom Oxyfuel CFB boilers: a promising option for CO2 capture [J].
Suraniti, Silvestre L. ;
Nsakala, Nsakala Ya ;
Darling, Scott L. .
GREENHOUSE GAS CONTROL TECHNOLOGIES 9, 2009, 1 (01) :543-548
[35]   Experiences and results on a 0.8 MWth oxy-fuel operation pilot-scale circulating fluidized bed [J].
Tan, Y. ;
Jia, L. ;
Wu, Y. ;
Anthony, E. J. .
APPLIED ENERGY, 2012, 92 :343-347
[36]   Oxy-fuel combustion of solid fuels [J].
Toftegaard, Maja B. ;
Brix, Jacob ;
Jensen, Peter A. ;
Glarborg, Peter ;
Jensen, Anker D. .
PROGRESS IN ENERGY AND COMBUSTION SCIENCE, 2010, 36 (05) :581-625
[37]   Pyrolysis and combustion characteristics of coals in oxyfuel combustion [J].
Wang, Chang'an ;
Zhang, Xiaoming ;
Liu, Yinhe ;
Che, Defu .
APPLIED ENERGY, 2012, 97 :264-273
[38]   NOx formation and reduction mechanisms in staged O2/CO2 combustion [J].
Watanabe, Hirotatsu ;
Yamamoto, Jun-ichiro ;
Okazaki, Ken .
COMBUSTION AND FLAME, 2011, 158 (07) :1255-1263
[39]   Characterization of ashes from a 100 kWth pilot-scale circulating fluidized bed with oxy-fuel combustion [J].
Wu, Yinghai ;
Wang, Chunbo ;
Tan, Yewen ;
Jia, Lufei ;
Anthony, Edward J. .
APPLIED ENERGY, 2011, 88 (09) :2940-2948