Turbulent flows in highly elastic wormlike micelles

被引:38
作者
Beaumont, Julien [1 ]
Louvet, Nicolas [1 ]
Divoux, Thibaut [2 ]
Fardin, Marc-Antoine [3 ]
Bodiguel, Hugues [1 ]
Lerouge, Sandra [3 ]
Manneville, Sebastien [2 ,4 ]
Colin, Annie [1 ]
机构
[1] CNRS, UMR 5258, Lab Futur, Pessac, France
[2] Univ Lyon, CNRS, UMR 5672, Ecole Normale Super Lyon,Lab Phys, F-69364 Lyon 07, France
[3] Univ Paris Diderot, CNRS, UMR 7057, Lab Matiere & Syst Complexes, F-75205 Paris 13, France
[4] Inst Univ France, Paris, France
基金
欧洲研究理事会;
关键词
TAYLOR-COUETTE; INSTABILITIES; SURFACTANT; DYNAMICS; INTERFACE;
D O I
10.1039/c2sm26760h
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This work reports on an experimental study of elastic turbulence in a semi-dilute wormlike micelle system made of a highly elastic betaine surfactant solution. The temporal evolution of both rheological quantities and local flow properties is monitored by combining global rheology, optical visualization, and ultrasonic velocimetry. Even at the smallest applied shear rates or shear stresses, we find that the micellar sample develops large Weissenberg (Wi) numbers, leading the flow to undergo a transition to elastic turbulence. Three-dimensional flows are indeed observed all along the flow curve, which therefore cannot be interpreted in the framework of classical shear banding. Strong fluctuations are also recorded in the rheological quantities, in the reflected light intensity, and in velocity profiles. We show that the power spectral densities (PSDs) of these fluctuations display power law behaviours with exponents ranging from -1 to -3 depending on the applied shear stress or shear rate. The exponents inferred from local velocity measurements are found to be spatially dependent, pointing to inhomogeneous turbulence. The nature of the instability and of the transition to elastic turbulence is further discussed in light of recent experimental and theoretical works on wormlike micelles and polymers.
引用
收藏
页码:735 / 749
页数:15
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