First field test of linear gas sensor net for planar detection of CO2 leakages in the unsaturated zone

被引:12
作者
Lazik, Detlef [1 ]
Ebert, Sebastian [1 ]
机构
[1] UFZ Helmholtz Ctr Environm Res, Dept Soil Phys, D-06198 Halle, Germany
关键词
Carbon capture and storage; Leakage; CO2; Gas sensor; Monitoring; Subsurface; WESTERN EGER RIFT; VADOSE ZONE; SOIL; SEEPAGE; CALDERA; STORAGE;
D O I
10.1016/j.ijggc.2013.04.014
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Gases from subsurface sources can present risks for the biosphere. To extend the lead time in managing such risks, reliable gas detection in the subsurface is required. A monitoring system was developed that is able to: (i) gather information from large areas, (ii) work efficiently within the subsurface; insensitive to changing subsurface environmental conditions while sensitive to changes in target gas concentrations, and (iii) provide a fast response. We report the first field test of linear membrane-based gas sensors: Fourteen 40 m long sensors were installed in two horizontal nets one above the other within a homogenized soil and scanned from a control station. 10 L/min of CO2 was injected into a point-like port 25 cm below the lower sensor net. Two operation modes were successfully tested to detect the CO2 plume: an active mode, which is sensitive to the concentration, and a passive mode, which is sensitive to changes in concentration. By conversion of the monitoring results the minimum contact range of seeping gas and sensor could be determined. Based on this valuable approach, an unexpectedly high level of lateral gas spread within the soil and the formation of a gas pillow below the soil surface could be observed. (C) 2013 Elsevier Ltd. All rights reserved.
引用
收藏
页码:161 / 169
页数:9
相关论文
共 33 条
[1]   Chernozem -: Soil of the Year 2005 [J].
Altermann, M ;
Rinklebe, J ;
Merbach, I ;
Körschens, M ;
Langer, U ;
Hofmann, B .
JOURNAL OF PLANT NUTRITION AND SOIL SCIENCE, 2005, 168 (06) :725-740
[2]   Gas migration along fault systems and through the vadose zone in the Latera caldera (central Italy):: Implications for CO2 geological storage [J].
Annunziatellis, A. ;
Beaubien, S. E. ;
Bigi, S. ;
Ciotoli, G. ;
Coltella, M. ;
Lombardi, S. .
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2008, 2 (03) :353-372
[3]   Short- and long-term gas hazard: the release of toxic gases in the Alban Hills volcanic area (central Italy) [J].
Annunziatellis, A ;
Ciotoli, G ;
Lombardi, S ;
Nolasco, F .
JOURNAL OF GEOCHEMICAL EXPLORATION, 2003, 77 (2-3) :93-108
[4]  
Bartholmai M., 2013, ENERGY PROC IN PRESS
[5]   Monthly monitoring of gas and isotope compositions in the free gas phase at degassing locations close to the Novy Kostel focal zone in the western Eger Rift, Czech Republic [J].
Braeuer, Karin ;
Kaempf, Horst ;
Koch, Ulrich ;
Strauch, Gerhard .
CHEMICAL GEOLOGY, 2011, 290 (3-4) :163-176
[6]  
Brandrup J., 1999, Polymer Handbook, VII
[7]   Modeling the effects of topography and wind on atmospheric dispersion of CO2 surface leakage at geologic carbon sequestration sites [J].
Chow, Fotini K. ;
Granvold, Patrick W. ;
Oldenburg, Curtis M. .
GREENHOUSE GAS CONTROL TECHNOLOGIES 9, 2009, 1 (01) :1925-1932
[8]   The role of optimality in characterizing CO2 seepage from geologic carbon sequestration sites [J].
Cortis, Andrea ;
Oldenburg, Curtis M. ;
Benson, Sally M. .
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2008, 2 (04) :640-652
[9]   Density-Corrected Models for Gas Diffusivity and Air Permeability in Unsaturated Soil [J].
Deepagoda, T. K. K. Chamindu ;
Moldrup, Per ;
Schjonning, Per ;
de Jonge, Lis Wollesen ;
Kawamoto, Ken ;
Komatsu, Toshiko .
VADOSE ZONE JOURNAL, 2011, 10 (01) :226-238
[10]   State-of-the-art Adsorption and Membrane Separation Processes for Carbon Dioxide Production from Carbon Dioxide Emitting Industries [J].
Ebner, Armin D. ;
Ritter, James A. .
SEPARATION SCIENCE AND TECHNOLOGY, 2009, 44 (06) :1273-1421