Hydrogenated Graphene as Metal-free Catalyst for Fenton-like Reaction

被引：21
作者：
Zhao, Yi
Chen, Wu-feng
Yuan, Cheng-fei
Zhu, Zi-ye
Yan, Li-feng [1 ]
机构：
[1] Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Peoples R China
来源：
CHINESE JOURNAL OF CHEMICAL PHYSICS | 2012年 / 25卷 / 03期
基金：
中国国家自然科学基金;
关键词：
Graphene; Hydrogenation; Metal-free; Catalysis; REVERSIBLE HYDROGENATION; REDUCTION; GRAPHITE; OXIDE; OXIDATION; CARBON; FILMS;
D O I：
10.1088/1674-0068/25/03/335-338
中图分类号：
O64 [物理化学（理论化学）、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号：
070203 ; 070304 ; 081704 ; 1406 ;
摘要：
Carbonaceous catalysts are potential alternatives to metal catalysts. Graphene has been paid much attention for its high surface area and light weight. Here, hydrogenated graphene has been prepared by a simple gamma ray irradiation of graphene oxide aqueous suspension at room temperature. Transmission electron microscopic, element analysis, X-ray photoelectron spectroscopy, and IN-Vis spectrophotometer studies verified the hydrogenation of graphene. The as-prepared hydrogenated graphene can be used as a metal-free carbonaceous catalyst for the Fenton-like degradation of organic dye in water.
引用
收藏
页码：335 / 338
页数：4
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  • [1] Electric field: A catalyst for hydrogenation of graphene
    Ao, Z. M.
    Peeters, F. M.
    [J]. APPLIED PHYSICS LETTERS, 2010, 96 (25)
  • [2] Evaluation of solution-processed reduced graphene oxide films as transparent conductors
    Becerril, Hdctor A.
    Mao, Jie
    Liu, Zunfeng
    Stoltenberg, Randall M.
    Bao, Zhenan
    Chen, Yongsheng
    [J]. ACS NANO, 2008, 2 (03) : 463 - 470
  • [3] XPS studies of graphite electrode materials for lithium ion batteries
    Blyth, RIR
    Buqa, H
    Netzer, FP
    Ramsey, MG
    Besenhard, JO
    Golob, P
    Winter, M
    [J]. APPLIED SURFACE SCIENCE, 2000, 167 (1-2) : 99 - 106
  • [4] Efficient preparation of highly hydrogenated graphene and its application as a high-performance anode material for lithium ion batteries
    Chen, Wufeng
    Zhu, Zhiye
    Li, Sirong
    Chen, Chunhua
    Yan, Lifeng
    [J]. NANOSCALE, 2012, 4 (06) : 2124 - 2129
  • [5] Preparation of graphene by a low-temperature thermal reduction at atmosphere pressure
    Chen, Wufeng
    Yan, Lifeng
    [J]. NANOSCALE, 2010, 2 (04) : 559 - 563
  • [6] Preparation of graphene by the rapid and mild thermal reduction of graphene oxide induced by microwaves
    Chen, Wufeng
    Yan, Lifeng
    Bangal, Prakriti R.
    [J]. CARBON, 2010, 48 (04) : 1146 - 1152
  • [7] Synthesis of graphene paper from pyrolyzed asphalt
    Cheng, I. Francis
    Xie, Yuqun
    Gonzales, R. Allen
    Brejna, Przemyslaw R.
    Sundararajan, Jency Pricilla
    Kengne, B. A. Fouetio
    Aston, D. Eric
    McIlroy, David N.
    Foutch, Jeremy D.
    Griffiths, Peter R.
    [J]. CARBON, 2011, 49 (08) : 2852 - 2861
  • [8] Electronic structure and transport properties of hydrogenated graphene and graphene nanoribbons
    Choe, D. H.
    Bang, Junhyeok
    Chang, K. J.
    [J]. NEW JOURNAL OF PHYSICS, 2010, 12
  • [9] Converting carbohydrates to bulk chemicals and fine chemicals over heterogeneous catalysts
    Climent, Maria J.
    Corma, Avelino
    Iborra, Sara
    [J]. GREEN CHEMISTRY, 2011, 13 (03) : 520 - 540
  • [10] Graphene Oxide: A Convenient Carbocatalyst for Facilitating Oxidation and Hydration Reactions
    Dreyer, Daniel R.
    Jia, Hong-Peng
    Bielawski, Christopher W.
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (38) : 6813 - 6816
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