Highly Transparent and Conductive Films of Densely Aligned Ultrathin Au Nanowire Monolayers

被引:114
作者
Sanchez-Iglesias, Ana [2 ,3 ]
Rivas-Murias, Beatriz [1 ]
Grzelczak, Marek [2 ,3 ,4 ]
Perez-Juste, Jorge [2 ]
Liz-Marzan, Luis M. [2 ,3 ,4 ]
Rivadulla, Francisco [1 ]
Correa-Duarte, Miguel A. [2 ]
机构
[1] Univ Santiago Compostela, Ctr Invest Quim Biolox & Mat Mol CIQUS, Santiago De Compostela 15782, Spain
[2] Univ Vigo, Dept Quim Fis, Vigo 36310, Spain
[3] CIC BiomaGUNE, Donostia San Sebastian 20009, Spain
[4] Basque Fdn Sci, Ikerbasque, Bilbao 48011, Spain
关键词
Gold nanowires; transparent electrodes; self-assembly; solution process; SILVER NANOWIRES; GOLD NANOWIRES; GRAPHENE FILMS; SOLAR-CELLS; DEPOSITION; NETWORKS; STATE;
D O I
10.1021/nl3021522
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The combination of low electrical resistance and high optical transparency in a single material is very uncommon. Developing these systems is a scientific challenge and a technological need, to replace ITO in flexible electronic components and other highly demanding applications. Here we report a facile method to prepare single layers of densely aligned ultrathin Au-nanowires, homogeneous over cm(2) areas. The as-deposited films show an electrical/optical performance competitive with ITO and graphene-based electrodes. Moreover, the Au-films show a good stability under ambient conditions, and the large aspect ratio of the ultrathin nanowires makes them perfect for deposition in flexible substrates.
引用
收藏
页码:6066 / 6070
页数:5
相关论文
共 31 条
[1]  
Andersson A, 1998, ADV MATER, V10, P859, DOI 10.1002/(SICI)1521-4095(199808)10:11<859::AID-ADMA859>3.0.CO
[2]  
2-1
[3]   Transparent Metal Nanowire Thin Films Prepared in Mesostructured Templates [J].
Azulai, Daniel ;
Belenkova, Tatyana ;
Gilon, Hagit ;
Barkay, Zahava ;
Markovich, Gil .
NANO LETTERS, 2009, 9 (12) :4246-4249
[4]   Solid-state dye-sensitized mesoporous TiO2 solar cells with high photon-to-electron conversion efficiencies [J].
Bach, U ;
Lupo, D ;
Comte, P ;
Moser, JE ;
Weissörtel, F ;
Salbeck, J ;
Spreitzer, H ;
Grätzel, M .
NATURE, 1998, 395 (6702) :583-585
[5]  
Bae S, 2010, NAT NANOTECHNOL, V5, P574, DOI [10.1038/nnano.2010.132, 10.1038/NNANO.2010.132]
[6]   Kinetically driven self assembly of highly ordered nanoparticle monolayers [J].
Bigioni, TP ;
Lin, XM ;
Nguyen, TT ;
Corwin, EI ;
Witten, TA ;
Jaeger, HM .
NATURE MATERIALS, 2006, 5 (04) :265-270
[7]   Insulating State and Breakdown of Fermi Liquid Description in Molecular-Scale Single-Crystalline Wires of Gold [J].
Chandni, U. ;
Kundu, Paromita ;
Singh, Abhishek K. ;
Ravishankar, N. ;
Ghosh, Arindam .
ACS NANO, 2011, 5 (10) :8398-8403
[8]   Continuous, Highly Flexible, and Transparent Graphene Films by Chemical Vapor Deposition for Organic Photovoltaics [J].
De Arco, Lewis Gomez ;
Zhang, Yi ;
Schlenker, Cody W. ;
Ryu, Koungmin ;
Thompson, Mark E. ;
Zhou, Chongwu .
ACS NANO, 2010, 4 (05) :2865-2873
[9]   Binary nanocrystal superlattice membranes self-assembled at the liquid-air interface [J].
Dong, Angang ;
Chen, Jun ;
Vora, Patrick M. ;
Kikkawa, James M. ;
Murray, Christopher B. .
NATURE, 2010, 466 (7305) :474-477
[10]   Simple and rapid synthesis of ultrathin gold nanowires, their self-assembly and application in surface-enhanced Raman scattering [J].
Feng, Huajun ;
Yang, Yanmei ;
You, Yumeng ;
Li, Gongping ;
Guo, Jun ;
Yu, Ting ;
Shen, Zexiang ;
Wu, Tom ;
Xing, Bengang .
CHEMICAL COMMUNICATIONS, 2009, (15) :1984-1986