Computer simulations of laser-induced melting of aluminum

Laser-induced solid-to-liquid phase transitions in 100 nm aluminum film were simulated using a hybrid model that combines molecular dynamics (MD) with a continuum description of the laser excitation and a two-temperature method (TTM) to model the relaxation of conduction band electrons. When the laser fluence provides more energy than needed for a complete melting of the film, the phase transition is characterized by an ultrafast collapse of the crystal structure within 2-3 ps. Otherwise, the transition involves a homogeneous nucleation and growth of liquid zones inside the crystal and a heterogeneous propagation of transition fronts from the external surfaces or nucleated liquid zones. (C) 2013 Elsevier B.V. All rights reserved.