Acceleration of Trimethylamine Removal Process Under Synergistic Effect of Photocatalytic Oxidation and Surface Discharge Plasma Reactor

被引:19
作者
Assadi, Aymen Amine [1 ,2 ]
Bouzaza, Abdelkrim [1 ,2 ]
Lemasle, Marguerite [1 ,2 ]
Wolbert, Dominique [1 ,2 ]
机构
[1] CNRS, UMR 6226, Equipe Chim & Ingn Proc, ENSCR 11,Lab Sci Chim Rennes, F-35708 Rennes, France
[2] Univ Europeenne Bretagne, Rennes, France
关键词
continuous reactor; synergetic effect; plasma/photocatalysis coupling; by-products identification; NONTHERMAL PLASMA; CATALYSTS; GAS; ADSORPTION; VAPOR;
D O I
10.1002/cjce.22211
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Removal of trimethylamine (TMA) from the air is experimentally investigated by combining photocatalysis with a DBD plasma reactor, at ambient temperature and atmospheric pressure. Many parameters are investigated in this work, such as flowrate, inlet concentration, relative humidity of effluent, and specific energy of discharge. By combining non-thermal plasma and photocatalysis, a synergy effect on the removal efficiency of TMA has been observed under different experimental conditions. Moreover, we note that adding a photocatalyst in the zone of plasma inhibits ozone formation. The formation of by-products due to TMA removal is also studied. The identified and analyzed by-products are classified into four groups: intermediary products, carbon monoxide, carbon dioxide, and ozone and nitrogen oxides.
引用
收藏
页码:1239 / 1246
页数:8
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