Research on aerosol sources and chemical composition: Past, current and emerging issues

被引：301

作者：

Calvo, A. I. ^{[1
]}

Alves, C. ^{[1
]}

Castro, A. ^{[2
]}

Pont, V. ^{[3
]}

Vicente, A. M. ^{[1
]}

Fraile, R. ^{[2
]}

机构：

[1] Univ Aveiro, Ctr Environm & Marine Studies CESAM, P-3810193 Aveiro, Portugal

[2] Univ Leon, IMARENAB, Dept Phys, E-24071 Leon, Spain

[3] Univ Toulouse 3, CNRS UPS, UMR 5550, Lab Aerol OMP, F-31400 Toulouse, France

来源：

ATMOSPHERIC RESEARCH | 2013年 / 120卷

关键词：

Aerosols; Historical aspects; Chemical composition; Sources; Research perspectives; SECONDARY ORGANIC AEROSOL; POLYCYCLIC AROMATIC-HYDROCARBONS; BIOMASS BURNING AEROSOL; EXHAUST PARTICULATE MATTER; SULFUR-DIOXIDE EMISSIONS; REGIONAL AIR-QUALITY; FIRED POWER-STATION; SOURCE APPORTIONMENT; CARBONACEOUS AEROSOLS; SIZE DISTRIBUTION;

D O I：

10.1016/j.atmosres.2012.09.021

中图分类号：

P4 [大气科学（气象学）];

学科分类号：

0706 ; 070601 ;

摘要：

In spite of considerable progresses in recent years, a quantitative and predictive understanding of atmospheric aerosol sources, chemical composition, transformation processes and environmental effects is still rather limited, and therefore represents a major research challenge in atmospheric science. This review begins with a historical perspective on the scientific questions regarding atmospheric aerosols over the past centuries, followed by a description of the distribution, sources, transformation processes, and chemical and physical properties as they are currently understood. The major open questions and suggestions for future research priorities are outlined to narrow the gap between the present understanding of the contribution of both anthropogenic and biogenic aerosols to radiative forcing resulting from the spatial non-uniformity, intermittency of sources, unresolved composition and reactivity. (C) 2012 Elsevier B.V. All rights reserved.

引用

页码：1 / 28

页数：28

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