Magnetic interactions in TDAE-C-60

被引:11
作者
Asai, Y [1 ]
Tokumoto, M [1 ]
Tanaka, K [1 ]
Sato, T [1 ]
Yamabe, T [1 ]
机构
[1] KYOTO UNIV, DIV MOLEC ENGN, KYOTO 60601, JAPAN
关键词
D O I
10.1103/PhysRevB.53.4176
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have introduced the two-channel Sherrington-Kirkpatrick (SK) model to account for the temperature dependency of the magnetization of TDAE-C-60 measured under very small magnetic field of order of 0.1 Oc. The two-channel SK model includes another glassy degree of freedom than spins. The second glassy degree of freedom couples to spins and hence has influence on the magnetic properties. This model is successful in explaining the rapid increase of the field cooling (FC) magnetization in the low-temperature region below the freezing temperature as well as the onset of the remanence, the difference between the FC and zero-field cooling magnetization, found in the experiment, both of which are difficult to explain simultaneously by the standard spin-glass models or ferromagnetic domains. While the phase in the two-channel SK model we found relevant for the experiment is quite different from the standard spin-glass models in the meaning described above, it has a similarity with the mixed phase of the SK model, in the meaning that both the Edward-Anderson order parameter and the spontaneous magnetization have nonzero values. This does not contradict the muon-spin-relaxation experiment, which shows the existence of the spontaneous magnetization in TDAE-C-60. We have also discussed the possible microscopic origin of the second glassy degree of freedom.
引用
收藏
页码:4176 / 4179
页数:4
相关论文
共 32 条
[1]   ORGANIC MOLECULAR SOFT FERROMAGNETISM IN A FULLERENE-C60 [J].
ALLEMAND, PM ;
KHEMANI, KC ;
KOCH, A ;
WUDL, F ;
HOLCZER, K ;
DONOVAN, S ;
GRUNER, G ;
THOMPSON, JD .
SCIENCE, 1991, 253 (5017) :301-303
[2]   ADIABATIC AND NONADIABATIC ELECTRON INTRAMOLECULAR-VIBRATION COUPLINGS AND SUPERCONDUCTIVITY IN FULLERENES [J].
ASAI, Y ;
KAWAGUCHI, Y .
PHYSICAL REVIEW B, 1992, 46 (02) :1265-1268
[3]   REDUCED-DENSITY-MATRIX ANALYSIS OF SUPERCONDUCTING CORRELATION IN 2-DIMENSIONAL AND 2-CHAIN HUBBARD MODELS [J].
ASAI, Y .
PHYSICAL REVIEW B, 1994, 50 (09) :6519-6522
[4]   ELEMENTARY-SPIN-EXCITATION SPECTRUM OF UNDOPED AND DOPED SINGLE-BAND HUBBARD MODELS [J].
ASAI, Y .
PHYSICAL REVIEW B, 1994, 49 (14) :10013-10015
[5]   JAHN-TELLER MECHANISM OF THE HALF WIDTH OF THE INTRAMOLECULAR VIBRATIONAL-SPECTRUM IN DOPED C60 - COUPLING WITH H(G), T(1U), AND H(U) MODES [J].
ASAI, Y .
PHYSICAL REVIEW B, 1994, 49 (06) :4289-4294
[6]   FERROMAGNETIC AND ANTIFERROMAGNETIC INTERMOLECULAR INTERACTIONS OF ORGANIC RADICALS, ALPHA-NITRONYL NITROXIDES .2. [J].
AWAGA, K ;
MARUYAMA, Y .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (04) :2743-2747
[7]   Structure and dynamics of crystalline C-60 [J].
Axe, JD ;
Moss, SC ;
Neumann, DA .
SOLID STATE PHYSICS - ADVANCES IN RESEARCH AND APPLICATIONS, VOL 48, 1994, 48 :149-224
[8]   TIME DECAY OF THE REMANENT MAGNETIZATION IN TDAE-C-60 [J].
BLINC, R ;
CEVC, P ;
ARCON, D ;
MIHAILOVIC, D ;
VENTURINI, P .
PHYSICAL REVIEW B, 1994, 50 (17) :13051-13053
[9]   POLARONS IN C60 [J].
FRIEDMAN, B .
PHYSICAL REVIEW B, 1992, 45 (03) :1454-1457
[10]   LATTICE AND ELECTRONIC-STRUCTURES OF UNDOPED AND DOPED C60 MOLECULES BY THE EXTENDED SU-SCHRIEFFER-HEEGER MODEL [J].
HARIGAYA, K .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1991, 60 (12) :4001-4004