Yb2Sn2O7: A magnetic Coulomb liquid at a quantum critical point

被引:26
作者
Dun, Z. L. [1 ]
Choi, E. S. [2 ]
Zhou, H. D. [1 ,2 ]
Hallas, A. M. [3 ]
Silverstein, H. J. [3 ]
Qiu, Y. [4 ,5 ]
Copley, J. R. D. [4 ]
Gardner, J. S. [4 ,6 ]
Wiebe, C. R. [2 ,3 ,7 ]
机构
[1] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA
[2] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32306 USA
[3] Univ Manitoba, Dept Chem, Winnipeg, MB R3T 2N2, Canada
[4] NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA
[5] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA
[6] Indiana Univ, Bloomington, IN 47408 USA
[7] Univ Winnipeg, Dept Chem, Winnipeg, MB R3B 2E9, Canada
基金
加拿大自然科学与工程研究理事会; 美国国家科学基金会;
关键词
SPIN ICE; MONOPOLES; TRANSITION;
D O I
10.1103/PhysRevB.87.134408
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report neutron scattering and ac susceptibility measurements on the pyrochlore Yb2Sn2O7. The appearance of magnetic diffuse scattering, low-energy spin excitations, and a nearly temperature-independent relaxation time are signatures that the system enters a short-range-ordered regime with quantum dynamics beneath 2 K. ac susceptibility data further suggest that Yb2Sn2O7 enters a long-range magnetically ordered state below 0.11 K. These results suggest that Yb(2)Sn(2)O7 is a ferromagnet with persistent spin dynamics down to 0.05 K. Referencing the phase diagram for Yb pyrochlores, Yb2Sn2O7 is approaching a quantum phase transition near the ferromagnetic ordered critical point. DOI: 10.1103/PhysRevB.87.134408
引用
收藏
页数:5
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共 37 条
[1]   Vindication of Yb2Ti2O7 as a Model Exchange Quantum Spin Ice [J].
Applegate, R. ;
Hayre, N. R. ;
Singh, R. R. P. ;
Lin, T. ;
Day, A. G. R. ;
Gingras, M. J. P. .
PHYSICAL REVIEW LETTERS, 2012, 109 (09)
[2]   HEAT-CAPACITY MEASUREMENTS ON RARE-EARTH DOUBLE OXIDES R2M2O7 [J].
BLOTE, HWJ ;
WIELINGA, RF ;
HUISKAMP, WJ .
PHYSICA, 1969, 43 (04) :549-&
[3]   Measurement of the charge and current of magnetic monopoles in spin ice [J].
Bramwell, S. T. ;
Giblin, S. R. ;
Calder, S. ;
Aldus, R. ;
Prabhakaran, D. ;
Fennell, T. .
NATURE, 2009, 461 (7266) :956-U211
[4]   Spin ice state in frustrated magnetic pyrochlore materials [J].
Bramwell, ST ;
Gingras, MJP .
SCIENCE, 2001, 294 (5546) :1495-1501
[5]   Bulk magnetization of the heavy rare earth titanate pyrochlores - a series of model frustrated magnets [J].
Bramwell, ST ;
Field, MN ;
Harris, MJ ;
Parkin, IP .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2000, 12 (04) :483-495
[6]   Ising versus XY Anisotropy in Frustrated R2Ti2O7 Compounds as "Seen'' by Polarized Neutrons [J].
Cao, H. ;
Gukasov, A. ;
Mirebeau, I. ;
Bonville, P. ;
Decorse, C. ;
Dhalenne, G. .
PHYSICAL REVIEW LETTERS, 2009, 103 (05)
[7]   Anisotropic exchange in frustrated pyrochlore Yb2Ti2O7 [J].
Cao, H. B. ;
Gukasov, A. ;
Mirebeau, I. ;
Bonville, P. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2009, 21 (49)
[8]   Magnetic monopoles in spin ice [J].
Castelnovo, C. ;
Moessner, R. ;
Sondhi, S. L. .
NATURE, 2008, 451 (7174) :42-45
[9]   Higgs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O7 [J].
Chang, Lieh-Jeng ;
Onoda, Shigeki ;
Su, Yixi ;
Kao, Ying-Jer ;
Tsuei, Ku-Ding ;
Yasui, Yukio ;
Kakurai, Kazuhisa ;
Lees, Martin Richard .
NATURE COMMUNICATIONS, 2012, 3
[10]   Dipolar interactions and origin of spin ice in Ising pyrochlore magnets [J].
den Hertog, BC ;
Gingras, MJP .
PHYSICAL REVIEW LETTERS, 2000, 84 (15) :3430-3433