Volcanic SO2 fluxes derived from satellite data: a survey using OMI, GOME-2, IASI and MODIS

被引:131
作者
Theys, N. [1 ]
Campion, R. [2 ]
Clarisse, L. [2 ]
Brenot, H. [1 ]
van Gent, J. [1 ]
Dils, B. [1 ]
Corradini, S. [3 ]
Merucci, L. [3 ]
Coheur, P. -F. [2 ]
Van Roozendael, M. [1 ]
Hurtmans, D. [2 ]
Clerbaux, C. [2 ,4 ]
Tait, S. [5 ]
Ferrucci, F. [5 ]
机构
[1] Belgian Inst Space Aeron BIRA IASB, Brussels, Belgium
[2] Univ Libre Bruxelles, Serv Chim Quant & Photophys, Brussels, Belgium
[3] INGV, Rome, Italy
[4] Univ Versailles St Quentin, Univ Paris 06, CNRS INSU, LATMOS IPSL, Paris, France
[5] IPGP, Paris, France
关键词
SULFUR-DIOXIDE FLUX; DISPERSION MODEL FLEXPART; NYAMURAGIRA VOLCANO; ATMOSPHERIC COMPOSITION; MIYAKEJIMA VOLCANO; AEROSOL LOAD; EMISSIONS; ERUPTION; GAS; STRATOSPHERE;
D O I
10.5194/acp-13-5945-2013
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Sulphur dioxide (SO2) fluxes of active degassing volcanoes are routinely measured with ground-based equipment to characterize and monitor volcanic activity. SO2 of unmonitored volcanoes or from explosive volcanic eruptions, can be measured with satellites. However, remote-sensing methods based on absorption spectroscopy generally provide integrated amounts of already dispersed plumes of SO2 and satellite derived flux estimates are rarely reported. Here we review a number of different techniques to derive volcanic SO2 fluxes using satellite measurements of plumes of SO2 and investigate the temporal evolution of the total emissions of SO2 for three very different volcanic events in 2011: Puyehue-Cordon Caulle (Chile), Nyamulagira (DR Congo) and Nabro (Eritrea). High spectral resolution satellite instruments operating both in the ultraviolet-visible (OMI/Aura and GOME-2/MetOp-A) and thermal infrared (IASI/MetOp-A) spectral ranges, and multispectral satellite instruments operating in the thermal infrared (MODIS/Terra-Aqua) are used. We show that satellite data can provide fluxes with a sampling of a day or less (few hours in the best case). Generally the flux results from the different methods are consistent, and we discuss the advantages and weaknesses of each technique. Although the primary objective of this study is the calculation of SO2 fluxes, it also enables us to assess the consistency of the SO2 products from the different sensors used.
引用
收藏
页码:5945 / 5968
页数:24
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