Titanium carbide Ti3C2Tx (MXene) enhanced PAN nanofiber membrane for air purification

被引:123
作者
Gao, Xue [1 ]
Li, Zhong-Kun [1 ]
Xue, Jian [1 ,2 ]
Qian, Yong [1 ]
Zhang, Li-Zhi [1 ]
Caro, Juergen [3 ]
Wang, Haihui [1 ]
机构
[1] South China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China
[2] South China Univ Technol, State Key Lab Pulp & Paper Engn, 381 Wushan Rd, Guangzhou 510640, Guangdong, Peoples R China
[3] Leibniz Univ Hannover, Inst Phys Chem & Electrochem, Callinstr 3A, D-30167 Hannover, Germany
关键词
MXene nanosheets; Air purification membrane; Antibacterial; PM2.5; Polyacrylonitrile nanofibers; ANTIBACTERIAL PROPERTIES; PM2.5; SEPARATION; MORTALITY; POLLUTION; AEROSOLS; BACTERIA; REMOVAL; FILTERS;
D O I
10.1016/j.memsci.2019.05.058
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Highly effective air filters are needed because of the increasing harm caused by air particulate matter pollution. Herein, two-dimensional titanium carbide Ti3C2Tx MXene nanosheets with active surface-terminating groups (O, OH and F) were used to modify the polyacrylonitrile (PAN) nanofiber filters to strengthen their interaction force with PM2.5. These forces were measured quantitatively through the force-distance curve-based AFM showing that the MXene modification of the PAN fiber induces three times larger interaction forces than before. The obtained filters show high PM2.5 removal efficiency of similar to 99.7% with a low pressure drop of similar to 42 Pa. Moreover, the presence of MXene nanosheets strongly inhibits the propagation of bacteria (e.g. E. coli and S. aureus) in the filters. Such filters can significantly improve air quality, especially in public places such as hospitals.
引用
收藏
页码:162 / 169
页数:8
相关论文
共 48 条
  • [1] 2D metal carbides and nitrides (MXenes) for energy storage
    Anasori, Babak
    Lukatskaya, Maria R.
    Gogotsi, Yury
    [J]. NATURE REVIEWS MATERIALS, 2017, 2 (02):
  • [2] An Estimate of the Global Burden of Anthropogenic Ozone and Fine Particulate Matter on Premature Human Mortality Using Atmospheric Modeling
    Anenberg, Susan C.
    Horowitz, Larry W.
    Tong, Daniel Q.
    West, J. Jason
    [J]. ENVIRONMENTAL HEALTH PERSPECTIVES, 2010, 118 (09) : 1189 - 1195
  • [3] [Anonymous], 2018, ADV MAT
  • [4] [Anonymous], ENV AEROSOL PHYS
  • [5] Ambient PM2.5 Reduces Global and Regional Life Expectancy
    Apte, Joshua S.
    Brauer, Michael
    Cohen, Aaron J.
    Ezzati, Majid
    Pope, C. Arden, III
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS, 2018, 5 (09): : 546 - 551
  • [6] Washable Multilayer Triboelectric Air Filter for Efficient Particulate Matter PM2.5 Removal
    Bai, Yu
    Han, Chang Bao
    He, Chuan
    Gu, Guang Qin
    Nie, Jin Hui
    Shao, Jia Jia
    Xiao, Tian Xiao
    Deng, Chao Ran
    Wang, Zhong Lin
    [J]. ADVANCED FUNCTIONAL MATERIALS, 2018, 28 (15)
  • [7] Study on PM2.5 pollution and the mortality due to lung cancer in China based on geographic weighted regression model
    Cao, Qilong
    Rui, Guoqiang
    Liang, Ying
    [J]. BMC PUBLIC HEALTH, 2018, 18
  • [8] FILTRATION OF AEROSOLS BY FIBROUS MEDIA
    CHEN, CY
    [J]. CHEMICAL REVIEWS, 1955, 55 (03) : 595 - 623
  • [9] Highly Stable and Antibacterial Two-Dimensional Tungsten Disulfide Lamellar Membrane for Water Filtration
    Cheng, Peng
    Chen, Yan
    Yan, Xi
    Wang, Yanjie
    Lang, Wan-Zhong
    [J]. CHEMSUSCHEM, 2019, 12 (01) : 275 - 282
  • [10] Assessing PM2.5 Exposures with High Spatiotemporal Resolution across the Continental United States
    Di, Qian
    Kloog, Itai
    Koutrakis, Petros
    Lyapustin, Alexei
    Wang, Yujie
    Schwartz, Joel
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2016, 50 (09) : 4712 - 4721