Size-Specific Spin Configurations in Single Iron Nanomagnet: From Flower to Exotic Vortices

被引:64
作者
Gatel, Christophe [1 ]
Bonilla, Francisco Javier [2 ,3 ]
Meffre, Anca [2 ,3 ]
Snoeck, Etienne [1 ]
Warot-Fonrose, Benedicte [1 ]
Chaudret, Bruno [2 ,3 ]
Lacroix, Lise-Marie [2 ,3 ]
Blon, Thomas [2 ,3 ]
机构
[1] CNRS, CEMES, F-31055 Toulouse, France
[2] Univ Toulouse, Lab Phys & Chim Nanoobjets, INSA UPS CNRS UMR5215, LPCNO, F-31077 Toulouse, France
[3] Inst Natl Sci Appl, F-31077 Toulouse, France
关键词
magnetic configuration; electron holography; vortex state; single domain state; flower state; nanocube; MAGNETIC DOMAIN-WALL; PARTICLES; GROWTH;
D O I
10.1021/acs.nanolett.5b02892
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The different spin configurations in the vicinity of the single-domain/vortex transition are reported in isolated magnetic nanoparticles. By combining chemical synthesis, electron holography in a dedicated transmission electron microscope and micromagnetic simulations, we establish the "magnetic configurations vs size" phase diagram of Fe single-crystalline nanocubes. Room temperature high resolution magnetic maps reveal the transition between single-domain and vortex states for Fe nanocubes from 25 to 27 nm, respectively. An intermediate spin configuration consisting of an < 111 > vortex is for the first time evidenced.
引用
收藏
页码:6952 / 6957
页数:6
相关论文
共 31 条
[1]   Off-axis electron holography of ferromagnetic multilayer nanowires [J].
Akhtari-Zavareh, Azadeh ;
Carignan, L. P. ;
Yelon, A. ;
Menard, D. ;
Kasama, T. ;
Herring, R. ;
Dunin-Borkowski, R. E. ;
McCartney, M. R. ;
Kavanagh, K. L. .
JOURNAL OF APPLIED PHYSICS, 2014, 116 (02)
[2]   Controlling multidomain states to enable sub-10-nm magnetic force microscopy [J].
Amos, Nissim ;
Ikkawi, Rabee ;
Haddon, Robert ;
Litvinov, Dmitri ;
Khizroev, Sakhrat .
APPLIED PHYSICS LETTERS, 2008, 93 (20)
[3]   Phase diagram for magnetic nano-rings [J].
Beleggia, M ;
Lau, JW ;
Schofield, MA ;
Zhu, Y ;
Tandon, S ;
De Graef, M .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2006, 301 (01) :131-146
[4]   Vortex state in ferromagnetic nanoparticles [J].
Betto, Davide ;
Coey, J. M. D. .
JOURNAL OF APPLIED PHYSICS, 2014, 115 (17)
[5]   Imaging the Fine Structure of a Magnetic Domain Wall in a Ni Nanocylinder [J].
Biziere, Nicolas ;
Gatel, Christophe ;
Lassalle-Balier, Remy ;
Clochard, Marie Claude ;
Wegrowe, Jean Eric ;
Snoeck, Etienne .
NANO LETTERS, 2013, 13 (05) :2053-2057
[6]  
Donahue M. J., 1999, OOMMF Users Guide
[7]  
Gandha Kinjal., 2014, Scientific reports, V4, P1
[8]   Mapping magnetic fields of Fe3O4 nanosphere assemblies by electron holography [J].
He, Kai ;
Ma, Fei-Xiang ;
Xu, Cheng-Yan ;
Cumings, John .
JOURNAL OF APPLIED PHYSICS, 2013, 113 (17)
[9]   Finite element calculations on the single-domain limit of a ferromagnetic cube -: a solution to μMAG Standard Problem No. 3 [J].
Hertel, R ;
Kronmüller, H .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2002, 238 (2-3) :185-199
[10]   Monodisperse Magnetic Nanoparticles for Theranostic Applications [J].
Ho, Don ;
Sun, Xiaolian ;
Sun, Shouheng .
ACCOUNTS OF CHEMICAL RESEARCH, 2011, 44 (10) :875-882