Topological rearrangements and stress fluctuations in quasi-two-dimensional hopper flow of emulsions

被引:33
作者
Chen, Dandan [1 ]
Desmond, Kenneth W. [1 ]
Weeks, Eric R. [1 ]
机构
[1] Emory Univ, Dept Phys, Atlanta, GA 30322 USA
基金
美国国家科学基金会;
关键词
REARRANGING DISORDERED PATTERNS; 2-DIMENSIONAL FOAMS; GRANULAR-MATERIALS; ELASTICITY; PLASTICITY; DYNAMICS; FORCES;
D O I
10.1039/c2sm26023a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We experimentally study the shear flow of oil-in-water emulsion droplets in a thin sample chamber with a hopper shape. In this thin chamber, the droplets are quasi-2D in shape. The sample is at an area fraction above jamming and forced to flow with a constant flux rate. Stresses applied to a droplet from its neighbors deform the droplet outline, and this deformation is quantified to provide an ad hoc measure of the stress. As the sample flows through the hopper we see large fluctuations of the stress, similar in character to what has been seen in other flows of complex fluids. Periods of time with large decreases in stress are correlated with bursts of elementary rearrangement events ("T1 events" where four droplets rearrange). More specifically, we see a local relationship between these observations: a T1 event decreases the inter-droplet forces up to 3 droplet diameters away from the event. This directly connects microscopic structural changes to macroscopic fluctuations, and confirms theoretical pictures of local rearrangements influencing nearby regions. These local rearrangements are an important means of reducing and redistributing stresses within a flowing material.
引用
收藏
页码:10486 / 10492
页数:7
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