Lightweight UiO-66/cellulose aerogels constructed through self-crosslinking strategy for adsorption applications

被引:167
作者
Wang, Zhongguo [1 ]
Song, Lian [1 ]
Wang, Yaquan [1 ]
Zhang, Xiong-Fei [1 ]
Hao, Dandan [2 ]
Feng, Yi [1 ]
Yao, Jianfeng [1 ]
机构
[1] Nanjing Forestry Univ, Jiangsu Key Lab Chem & Utilizat Agr & Forest Biom, Jiangsu Coinnovat Ctr Efficient Proc & Utilizat F, Coll Chem Engn, Nanjing 210037, Jiangsu, Peoples R China
[2] Southeast Univ, Sch Chem & Chem Engn, Nanjing 211189, Jiangsu, Peoples R China
关键词
Aerogel; Nanocellulose; Water treatment; UiO-66; Self-crosslinking; GAS SEPARATION; COMPOSITE MEMBRANES; FRAMEWORK COMPOSITE; CELLULOSE AEROGELS; METAL; REMOVAL; GROWTH; NANOPARTICLES; TRANSPARENT; PERFORMANCE;
D O I
10.1016/j.cej.2019.04.022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Composite UiO-66/nanocellulose aerogels with hierarchical pores and low density were prepared through a self-crosslinking method. The nanocellulose acted as the structural skeleton supporting and dispersing the UiO-66 particles. The micropore and accessibility of UiO-66 were well-preserved, making the composite aerogels ideal sorbents for water purification. The composite aerogels demonstrated high adsorption ability towards both anionic methyl orange (71.7 mg g(-1)) and cationic methylene blue (51.8 mg g(-1)). This work holds a promise to rational design and fabrication of MOF monoliths through group linkage.
引用
收藏
页码:138 / 144
页数:7
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