On the origin of reactivity of steam reforming of ethylene glycol on supported Ni catalysts

被引:37
|
作者
Li, Shuirong [1 ]
Zhang, Chengxi [1 ]
Zhang, Peng [1 ]
Wu, Gaowei [1 ]
Ma, Xinbin [1 ]
Gong, Jinlong [1 ]
机构
[1] Tianjin Univ, Sch Chem Engn & Technol, Minist Educ, Key Lab Green Chem Technol, Tianjin 300072, Peoples R China
基金
中国国家自然科学基金;
关键词
HYDROGEN-PRODUCTION; RENEWABLE HYDROGEN; FUEL-CELLS; CONVERSION; CELLULOSE; ETHANOL; HYDROCARBONS; CHEMICALS; ALCOHOLS;
D O I
10.1039/c2cp24089k
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This paper describes a strategy for producing hydrogen via steam reforming of ethylene glycol over supported nickel catalysts. Nickel plays a crucial role in conversion of ethylene glycol and production of hydrogen, while oxide supports affect product distribution of carbonaceous species. A plausible reaction pathway is proposed based on our results and the literature.
引用
收藏
页码:4066 / 4069
页数:4
相关论文
共 50 条
  • [41] Stability and activity of carbon nanofiber-supported catalysts in the aqueous phase reforming of ethylene glycol
    T. van Haasterecht
    C. C. I. Ludding
    K. P. de Jong
    J. H. Bitter
    Journal of Energy Chemistry, 2013, 22 (02) : 257 - 269
  • [42] Stability and activity of carbon nanofiber-supported catalysts in the aqueous phase reforming of ethylene glycol
    van Haasterecht, T.
    Ludding, C. C. I.
    de Jong, K. P.
    Bitter, J. H.
    JOURNAL OF ENERGY CHEMISTRY, 2013, 22 (02) : 257 - 269
  • [43] Aqueous-phase reforming of ethylene glycol over supported Pt and Pd bimetallic catalysts
    Huber, GW
    Shabaker, JW
    Evans, ST
    Dumesic, JA
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2006, 62 (3-4) : 226 - 235
  • [44] Steam reforming and graphite formation on Ni catalysts
    Bengaard, HS
    Norskov, JK
    Sehested, J
    Clausen, BS
    Nielsen, LP
    Molenbroek, AM
    Rostrup-Nielsen, JR
    JOURNAL OF CATALYSIS, 2002, 209 (02) : 365 - 384
  • [45] Zircon supported copper catalysts for the steam reforming of methanol
    Widiastri, M.
    Fendy
    Marsih, I. N.
    NEUTRON AND X-RAY SCATTERING IN MATERIALS SCIENCE AND BIOLOGY, 2008, 989 : 248 - 251
  • [46] Study on steam reforming of naphthalene in presence of supported catalysts
    Yu, Yingmin
    PETROLEUM SCIENCE AND TECHNOLOGY, 2018, 36 (12) : 910 - 914
  • [47] Steam reforming of dodecane over supported iridium catalysts
    Ando, T
    Ikenaga, N
    Nakagawa, K
    Suzuki, T
    JOURNAL OF THE JAPAN PETROLEUM INSTITUTE, 2002, 45 (06) : 409 - 413
  • [48] Hydrogen production by steam reforming of n-butane over supported Ni and Pt-Ni catalysts
    Avci, AK
    Trimm, DL
    Aksoylu, AE
    Önsan, ZI
    APPLIED CATALYSIS A-GENERAL, 2004, 258 (02) : 235 - 240
  • [49] Glycerol steam reforming over Ni catalysts supported on ceria and ceria-promoted alumina
    Iriondo, A.
    Barrio, V. L.
    Cambra, J. F.
    Arias, P. L.
    Guemez, M. B.
    Sanchez-Sanchez, M. C.
    Navarro, R. M.
    Fierro, J. L. G.
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2010, 35 (20) : 11622 - 11633
  • [50] Characterization of alumina-supported Ni and Ni-Pd catalysts for partial oxidation and steam reforming of hydrocarbons
    Zhang, JC
    Wang, YH
    Ma, RY
    Wu, DY
    APPLIED CATALYSIS A-GENERAL, 2003, 243 (02) : 251 - 259