Synthesis of novel MoS2/g-C3N4nanocomposites for enhanced photocatalytic activity

被引:6
作者
Wei, Zhen [1 ]
Shen, Xiaoning [1 ]
Ji, Yongfeng [1 ]
Yang, Zhichao [1 ]
Wang, Tong [1 ]
Li, Shu [1 ]
Zhu, Menghan [2 ]
Tian, Ye [2 ]
机构
[1] Hebei North Univ, Coll Sci, Dept Chem, Zhangjiakou 075000, Peoples R China
[2] Hebei North Univ, Coll Sci, Dept Phys, Zhangjiakou 075000, Peoples R China
关键词
H-2; EVOLUTION; FACILE SYNTHESIS; G-C3N4; DEGRADATION; HYDROGEN; FABRICATION; MOS2; HETEROJUNCTION; PERFORMANCE; COMPOSITES;
D O I
10.1007/s10854-020-04150-8
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
So far, the synthesis of high-activity and low-cost photocatalysts remains a huge challenge. 3D flower-like MoS2/g-C(3)N(4)hybrids were synthesized by a very simple method. All of them were characterized by various characterizations to determine the composition, morphology, and properties of the compounds. There are many sites with large specific surface area catalytic activity in this structure. These composites are all photocatalytic degradable organic dyes, and the photocatalytic properties of the flower-like 4% MoS2/g-C(3)N(4)are the best. The stability and recyclability of the 4% MoS2/g-C(3)N(4)photocatalyst are also excellent. The 4% MoS2/g-C(3)N(4)can also have photocatalytic ability to produce hydrogen. 50 mg of 4% MoS2/g-C(3)N(4)photocatalyst can produce about 156 umol of hydrogen with visible light irradiation for about 4 h. Rate of hydrogen production is about 780 mu mol h(- 1) g(- 1). In view of the good photocatalytic performance of the catalyst, we have discussed the mechanism both photocatalytic degradation of organic harmful pollutants and photocatalytic hydrogen production.
引用
收藏
页码:15885 / 15895
页数:11
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