Turning a molecule into a coherent two-level quantum system

被引:132
作者
Wang, Daqing [1 ]
Kelkar, Hrishikesh [1 ]
Martin-Cano, Diego [1 ]
Rattenbacher, Dominik [1 ]
Shkarin, Alexey [1 ]
Utikal, Tobias [1 ]
Goetzinger, Stephan [1 ,2 ]
Sandoghdar, Vahid [1 ,2 ]
机构
[1] Max Planck Inst Sci Light, Erlangen, Germany
[2] Friedrich Alexander Univ, Dept Phys, Erlangen, Germany
关键词
SINGLE-MOLECULE; NONLINEAR OPTICS; PHOTON; ATOM; SPECTROSCOPY; CRYSTAL;
D O I
10.1038/s41567-019-0436-5
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The use of molecules in quantum optical applications has been hampered by incoherent internal vibrations and other phononic interactions with their environment. Here we show that an organic molecule placed into an optical microcavity behaves as a coherent two-level quantum system. This allows the observation of 99% extinction of a laser beam by a single molecule, saturation with less than 0.5 photons and non-classical generation of few-photons super-bunched light. Furthermore, we demonstrate efficient interaction of the molecule-microcavity system with single photons generated by a second molecule in a distant laboratory. Our achievements represent an important step towards linear and nonlinear quantum photonic circuits based on organic platforms.
引用
收藏
页码:483 / +
页数:8
相关论文
共 48 条
  • [1] Giant optical nonlinearity induced by a single two-level system interacting with a cavity in the Purcell regime
    Auffeves-Garnier, Alexia
    Simon, Christoph
    Gerard, Jean-Michel
    Poizat, Jean-Philippe
    [J]. PHYSICAL REVIEW A, 2007, 75 (05):
  • [2] Bennett AJ, 2016, NAT NANOTECHNOL, V11, P857, DOI [10.1038/NNANO.2016.113, 10.1038/nnano.2016.113]
  • [3] Berman P.R, 1994, Cavity Quantum Electrodynamics, Advances in atomic, molecular, and optical physics
  • [4] QUANTUM INTERFERENCE AND COLLAPSE OF THE WAVE-FUNCTION IN CAVITY QED
    CARMICHAEL, HJ
    BRECHA, RJ
    RICE, PR
    [J]. OPTICS COMMUNICATIONS, 1991, 82 (1-2) : 73 - 79
  • [5] Chang DE, 2014, NAT PHOTONICS, V8, P685, DOI [10.1038/nphoton.2014.192, 10.1038/NPHOTON.2014.192]
  • [6] Single-molecule strong coupling at room temperature in plasmonic nanocavities
    Chikkaraddy, Rohit
    de Nijs, Bart
    Benz, Felix
    Barrow, Steven J.
    Scherman, Oren A.
    Rosta, Edina
    Demetriadou, Angela
    Fox, Peter
    Hess, Ortwin
    Baumberg, Jeremy J.
    [J]. NATURE, 2016, 535 (7610) : 127 - 130
  • [7] Tuning the Fluorescence Emission Spectra of a Single Molecule with a Variable Optical Subwavelength Metal Microcavity
    Chizhik, Alexey
    Schleifenbaum, Frank
    Gutbrod, Raphael
    Chizhik, Anna
    Khoptyar, Dmitry
    Meixner, Alfred J.
    Enderlein, Joerg
    [J]. PHYSICAL REVIEW LETTERS, 2009, 102 (07)
  • [8] Quasieigenstate Coalescence in an Atom-Cavity Quantum Composite
    Choi, Youngwoon
    Kang, Sungsam
    Lim, Sooin
    Kim, Wookrae
    Kim, Jung-Ryul
    Lee, Jai-Hyung
    An, Kyungwon
    [J]. PHYSICAL REVIEW LETTERS, 2010, 104 (15)
  • [9] Cohen-Tannoudji C, 2004, ATOM PHOTON INTERACT
  • [10] Strongly coupling a cavity to inhomogeneous ensembles of emitters: Potential for long-lived solid-state quantum memories
    Diniz, I.
    Portolan, S.
    Ferreira, R.
    Gerard, J. M.
    Bertet, P.
    Auffeves, A.
    [J]. PHYSICAL REVIEW A, 2011, 84 (06):