Emission inventory evaluation using observations of regional atmospheric background stations of China

被引:21
作者
An, Xingqin [1 ]
Sun, Zhaobin [2 ]
Lin, Weili [1 ]
Jin, Min [1 ]
Li, Nan [1 ]
机构
[1] Chinese Acad Meteorol Sci, China Meteorol Adm, Beijing 100081, Peoples R China
[2] Beijing Meteorol Observ, Beijing 100089, Peoples R China
基金
中国国家自然科学基金;
关键词
evaluation; CMAQ model; INTEX-B2006; inventory; regional atmospheric background stations; CARBON EMISSIONS; SURFACE OZONE; BLACK CARBON; MODEL; POLLUTANTS; MISSION;
D O I
10.1016/S1001-0742(12)60082-5
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Any accurate simulation of regional air quality by numerical models entails accurate and up-to-date emissions data for that region. The INTEX-B2006 (I06), one of the newest emission inventories recently popularly used in China and East Asia, has been assessed using the Community Multiscale Air Quality model and observations from regional atmospheric background stations of China. Comparisons of the model results with the observations for the species SO2, NO2, O-3 and CO from the three regional atmospheric background stations of Shangdianzi, Longfengshan and Linan show that the model can basically capture the temporal characteristics of observations such as the monthly, seasonal and diurnal variance trends. Compared to the other three species, the simulated CO values were grossly underestimated by about two-third or one-half of the observed values, related to the uncertainty in CO emissions. Compared to the other two stations, Shangdianzi had poorer simulations, especially for SO2 and CO, which partly resulted from the site location close to local emission sources from the Beijing area; and the regional inventory used was not capable of capturing the influencing factors of strong regional sources on stations. Generally, the fact that summer gave poor simulation, especially for SO2 and O-3, might partly relate to poor simulations of meteorological fields such as temperature and wind.
引用
收藏
页码:537 / 546
页数:10
相关论文
共 20 条
[1]   Formal uncertainty analysis of a Lagrangian photochemical air pollution model [J].
Bergin, MS ;
Noblet, GS ;
Petrini, K ;
Dhieux, JR ;
Milford, JB ;
Harley, RA .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1999, 33 (07) :1116-1126
[2]   A technology-based global inventory of black and organic carbon emissions from combustion [J].
Bond, TC ;
Streets, DG ;
Yarber, KF ;
Nelson, SM ;
Woo, JH ;
Klimont, Z .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D14) :D14203
[3]   Review of the governing equations, computational algorithms, and other components of the models-3 Community Multiscale Air Quality (CMAQ) modeling system [J].
Byun, Daewon ;
Schere, Kenneth L. .
APPLIED MECHANICS REVIEWS, 2006, 59 (1-6) :51-77
[4]   Inventory of black carbon and organic carbon emissions from China [J].
Cao, Guoliang ;
Zhang, Xiaoye ;
Zheng, Fangcheng .
ATMOSPHERIC ENVIRONMENT, 2006, 40 (34) :6516-6527
[5]   Evaluating regional emission estimates using the TRACE-P observations [J].
Carmichael, GR ;
Tang, Y ;
Kurata, G ;
Uno, I ;
Streets, DG ;
Thongboonchoo, N ;
Woo, JH ;
Guttikunda, S ;
White, A ;
Wang, T ;
Blake, DR ;
Atlas, E ;
Fried, A ;
Potter, B ;
Avery, MA ;
Sachse, GW ;
Sandholm, ST ;
Kondo, Y ;
Talbot, RW ;
Bandy, A ;
Thorton, D ;
Clarke, AD .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D21)
[6]  
Grell G., 1994, NCAR TECH NOTE, P1
[7]   Monte Carlo estimates of uncertainties in predictions by a photochemical grid model (UAM-IV) due to uncertainties in input variables [J].
Hanna, SR ;
Chang, JC ;
Fernau, ME .
ATMOSPHERIC ENVIRONMENT, 1998, 32 (21) :3619-3628
[8]   Transport and Chemical Evolution over the Pacific (TRACE-P) aircraft mission: Design, execution, and first results [J].
Jacob, DJ ;
Crawford, JH ;
Kleb, MM ;
Connors, VS ;
Bendura, RJ ;
Raper, JL ;
Sachse, GW ;
Gille, JC ;
Emmons, L ;
Heald, CL .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D20) :1-19
[9]  
Jiang X.K., 2002, RES AIR POLLUTION CO, P1
[10]   Contributions of pollutants from north china plain to surface ozone at the shangdianzi GAW station [J].
Lin, W. ;
Xu, X. ;
Zhang, X. ;
Tang, J. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2008, 8 (19) :5889-5898