Microwave-assisted catalytic pyrolysis of moso bamboo for high syngas production

被引:64
作者
Dong, Qing [1 ]
Niu, Miaomiao [2 ]
Bi, Dongmei [3 ]
Liu, Weiyu [1 ]
Gu, Xuexin [1 ]
Lu, Chen [1 ]
机构
[1] Huaiyin Inst Technol, Sch Life Sci & Food Engn, Jiangsu Prov Engn Lab Biomass Convers & Proc Inte, Huaian 223003, Peoples R China
[2] Nanjing Inst Technol, Coll Energy & Power Engn, Nanjing 211167, Jiangsu, Peoples R China
[3] Shandong Univ Technol, Sch Agr Engn & Food Sci, Zibo 255049, Peoples R China
基金
美国国家科学基金会;
关键词
Microwaves; Pyrolysis; Activated carbon; Moso bamboo; Iron(III) ion; BIOMASS GASIFICATION; ANAEROBIC-DIGESTION; STEAM GASIFICATION; FLUIDIZED-BED; TAR; MICROALGAE; GENERATION; HYDROGEN; SUPPORT; CHARS;
D O I
10.1016/j.biortech.2018.02.018
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
Microwave-assisted pyrolysis of moso bamboo with the activated carbon-supported iron(III) ion catalyst was carried out with the aim of obtaining high quality and quantity syngas(H-2 + CO). The effect of the catalyst on moso bomboo pyrolysis involving the temperature-rising characteristics, product distribution, tar conversion and gas compositions were investigated. The results indicated that the catalyst improved the microwave-absorption capability and increased the maximum reaction temperatures. The formation of gases was promoted by the catalyst mainly at the expense of the tar, indicating the catalyst had an excellent activity for the tar conversion. The catalyst had the positive influence on the formation of syngas with the maximum content reaching up to 81.14 vol% with H-2/CO being 1.04 and inhibited the production of CH4 and CO2. The loading of iron(III) ion into activated carbon exerted a significant influence on bamboo pyrolysis. The addition of the catalyst increased the thermal efficiency of the reaction system.
引用
收藏
页码:145 / 151
页数:7
相关论文
共 35 条
[11]   The catalytic pyrolysis of microalgae to produce syngas [J].
Hu, Zhifeng ;
Ma, Xiaoqian ;
Li, Longjun ;
Wu, Jie .
ENERGY CONVERSION AND MANAGEMENT, 2014, 85 :545-550
[12]   A study on experimental characteristic of microwave-assisted pyrolysis of microalgae [J].
Hu, Zhifeng ;
Ma, Xiaoqian ;
Chen, Chunxiang .
BIORESOURCE TECHNOLOGY, 2012, 107 :487-493
[13]   Application of atmospheric pressure microwave plasma source for production of hydrogen via methane reforming [J].
Jasinski, M. ;
Dors, M. ;
Mizeraczyk, J. .
EUROPEAN PHYSICAL JOURNAL D, 2009, 54 (02) :179-183
[14]   Biofuel production from birch wood by combining high solid loading simultaneous saccharification and fermentation and anaerobic digestion [J].
Kalyani, Dayanand Chandrahas ;
Zamanzadeh, Mirzaman ;
Mueller, Gerdt ;
Horn, Svein J. .
APPLIED ENERGY, 2017, 193 :210-219
[15]   Development of Ni catalysts for tar removal by steam gasification of biomass [J].
Kimura, Takeo ;
Miyazawa, Tomohisa ;
Nishikawa, Jin ;
Kado, Shigeru ;
Okumura, Kazu ;
Miyao, Toshihiro ;
Naito, Shuichi ;
Kunimori, Kimio ;
Tomishige, Keiichi .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2006, 68 (3-4) :160-170
[16]   Thermochemical Biomass Gasification: A Review of the Current Status of the Technology [J].
Kumar, Ajay ;
Jones, David D. ;
Hanna, Milford A. .
ENERGIES, 2009, 2 (03) :556-581
[17]   Development of Ni-Fe bimetallic based catalysts for biomass tar cracking/reforming: Effects of catalyst support and co-fed reactants on tar conversion characteristics [J].
Laosiripojana, N. ;
Sutthisripok, W. ;
Charojrochkul, S. ;
Assabumrungrat, S. .
FUEL PROCESSING TECHNOLOGY, 2014, 127 :26-32
[18]   Biomass gasification in a circulating fluidized bed [J].
Li, XT ;
Grace, JR ;
Lim, CJ ;
Watkinson, AP ;
Chen, HP ;
Kim, JR .
BIOMASS & BIOENERGY, 2004, 26 (02) :171-193
[19]   Boosting biomethane yield and production rate with graphene: The potential of direct interspecies electron transfer in anaerobic digestion [J].
Lin, Richen ;
Cheng, Jun ;
Zhang, Jiabei ;
Zhou, Junhu ;
Cen, Kefa ;
Murphy, Jerry D. .
BIORESOURCE TECHNOLOGY, 2017, 239 :345-352
[20]   Microwave heating processes involving carbon materials [J].
Menendez, J. A. ;
Arenillas, A. ;
Fidalgo, B. ;
Fernandez, Y. ;
Zubizarreta, L. ;
Calvo, E. G. ;
Bermudez, J. M. .
FUEL PROCESSING TECHNOLOGY, 2010, 91 (01) :1-8