Realizing Maximum Microwave Absorption of Poly(3,4-ethylenedioxythiophene) with a Data-Driven Method

被引:23
作者
Green, Michael [1 ]
Anh Thi Van Tran [1 ]
Chen, Xiaobo [1 ]
机构
[1] Univ Missouri, Dept Chem, Kansas City, MO 64110 USA
基金
美国国家科学基金会;
关键词
band analysis; microwave absorption; conducting polymers; permittivity/permeability; data-driven methods; data modeling; FACILE SYNTHESIS; ABSORBING PROPERTIES; COMPOSITES; REFLECTION;
D O I
10.1021/acsaelm.0c00573
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Large reflection loss (RL) and broad effective bandwidth (Delta f(10)) are two of the most important parameters for microwave-absorbing materials (MAMs). In this article, we report that a strong and broad microwave absorption can be obtained with poly(3,4-ethylenedioxythiophene) (PEDOT), with record-setting values over previous studies. These record-setting values are derived using a data-driven method to optimize the response parameters. We demonstrate that RL values are achieved of -54.0 dB centering 8.3 GHz with 3.4 mm thick 30.0 wt % PEDOT film and -42.6 dB centering 17.0 GHz with 1.5 mm film for 40.0 wt % PEDOT; Delta f(10) values of 5.8 and 5.2 GHz are shown with a film thickness of 2.1 and 1.7 mm, respectively.
引用
收藏
页码:2937 / 2944
页数:8
相关论文
共 50 条
[31]   UV copper ion laser treatment of poly(3,4-ethylenedioxythiophene) [J].
Ilieva, M. ;
Tsakova, V. ;
Vuchkov, N. K. ;
Temelkov, K. A. ;
Sabotinov, N. V. .
JOURNAL OF OPTOELECTRONICS AND ADVANCED MATERIALS, 2007, 9 (02) :303-306
[32]   Direct local polymerization of poly(3,4-ethylenedioxythiophene) in rat cortex [J].
Ouyang, Liangqi ;
Green, Rylie ;
Feldman, Kathleen E. ;
Martin, David C. .
BRAIN MACHINE INTERFACES: IMPLICATIONS FOR SCIENCE, CLINICAL PRACTICE AND SOCIETY, 2011, 194 :263-271
[33]   Biocompatible Smart Matrices Based on Poly (3,4-ethylenedioxythiophene)-Poly (N-isopropylacrylamide) Composite [J].
Sharma, Ashok K. ;
Sharma, Yashpal ;
Duhan, Surender .
INTERNATIONAL JOURNAL OF POLYMERIC MATERIALS AND POLYMERIC BIOMATERIALS, 2015, 64 (07) :333-337
[34]   Fabrication of poly(vinyl alcohol)-graphene quantum dots coated with poly(3,4-ethylenedioxythiophene) for supercapacitor [J].
Abidin, Shariffah Nur Jannah Syed Zainol ;
Mamat, Shuhazlly ;
Rasyid, Suraya Abdul ;
Zainal, Zulkarnain ;
Sulaiman, Yusran .
JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY, 2018, 56 (01) :50-58
[35]   Poly(pyrrole) versus poly(3,4-ethylenedioxythiophene): amperometric cholesterol biosensor matrices [J].
Tuerkarslan, Oezlem ;
Kayahan, Senem Kiralp ;
Toppare, Levent .
JOURNAL OF SOLID STATE ELECTROCHEMISTRY, 2009, 13 (05) :657-663
[36]   Poly(pyrrole) versus poly(3,4-ethylenedioxythiophene): amperometric cholesterol biosensor matrices [J].
Özlem Türkarslan ;
Senem Kıralp Kayahan ;
Levent Toppare .
Journal of Solid State Electrochemistry, 2009, 13 :657-663
[37]   Design and synthesis of core-shell porous magnetic nanospindle@poly(3,4-ethylenedioxythiophene)/MXene composite for efficient microwave absorption [J].
Zhu, Yuying ;
Ling, Xin ;
Dong, Qian ;
Liu, Qinglei ;
Wu, Yu ;
Jin, Qingjun ;
Zhang, Wang .
JOURNAL OF MATERIALS SCIENCE, 2023, 58 (38) :15100-15115
[38]   Effects of Solvents on the Morphology and Conductivity of Poly(3,4-ethylenedioxythiophene):Poly(styrenesulfonate) Nanofibers [J].
Kara, Meryem O. Pehlivaner ;
Frey, Margaret W. .
JOURNAL OF APPLIED POLYMER SCIENCE, 2014, 131 (11)
[39]   Poly (3,4-ethylenedioxythiophene) (PEDOT) and poly (3,4-ethylenedioxythiophene)-few walled carbon nanotube (PEDOT-FWCNT) nanocomposite based thin films for Schottky diode application [J].
Gupta, Bhavana ;
Mehta, Minisha ;
Melvin, Ambrose ;
Kamalakannan, R. ;
Dash, S. ;
Kamruddin, M. ;
Tyagi, A. K. .
MATERIALS CHEMISTRY AND PHYSICS, 2014, 147 (03) :867-877
[40]   Electrosynthesis, characterization, and application of poly(3,4-ethylenedioxythiophene) derivative with a chloromethyl functionality [J].
Zhang, Long ;
Wen, Yangping ;
Yao, Yuanyuan ;
Duan, Xuemin ;
Xu, Jingkun ;
Wang, Xiaoqiang .
JOURNAL OF APPLIED POLYMER SCIENCE, 2013, 130 (04) :2660-2670