POCIS Calibration for Organic Compound Sampling in Small Headwater Streams

被引：10
作者：
Booij, Kees [1 ]
Chen, Sunmao [2 ]
Trask, Jennifer R. [3 ]
机构：
[1] Pass Sampling Organ Cpds PaSOC, Kimswerd, Netherlands
[2] Syngenta Crop Protect, Greensboro, NC USA
[3] Waterborne Environm, Leesburg, VA USA
来源：
ENVIRONMENTAL TOXICOLOGY AND CHEMISTRY | 2020年 / 39卷 / 07期
关键词：
Passive sampler; Herbicide; Pesticide runoff; Sampling rate; Temperature; Flow; CHEMICAL INTEGRATIVE SAMPLERS; IN-SITU; DIFFUSIVE GRADIENTS; POLAR COMPOUNDS; WATER; MEMBRANE; HYDRODYNAMICS; POLLUTANTS; RANGE;
D O I：
10.1002/etc.4731
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
Field-based atrazine sampling rates (R-s) obtained by the polar organic chemical integrative sampler (POCIS) method were measured in 9 headwater streams over 3 yr covering 5 to 6 exposure periods of 2 to 3 wk/site/yr. Rates were best in line with the model R-s = 148 mL/d, with a standard deviation of 0.17 log units (factor 1.5). The POCIS canisters reduced mass transfer coefficients of the water boundary layer by a factor of 2 as measured by alabaster dissolution rates. A mechanistic model that accounts for flow and temperature effects yielded a fair estimate of the effective exchange surface area (12.5 +/- 0.8 cm(2)). This model could only be tested for higher flow velocities because of uncertainties associated with the measurement of flow velocities Environ Toxicol Chem 2020;00:1-9. (c) 2020 SETAC
引用
收藏
页码：1334 / 1342
页数：9
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