Exchange energy dominated by large orbital spin-currents in δ-Pu

被引:19
作者
Cricchio, Francesco [1 ]
Bultmark, Fredrik [1 ]
Nordstrom, Lars [1 ]
机构
[1] Uppsala Univ, Dept Phys & Mat Sci, SE-75121 Uppsala, Sweden
来源
PHYSICAL REVIEW B | 2008年 / 78卷 / 10期
基金
瑞典研究理事会;
关键词
D O I
10.1103/PhysRevB.78.100404
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The electronic structure of the anomalous delta phase of Pu is analyzed by a general and exact reformulation of the exchange energy of the f shell. It is found that the dominating contribution to the exchange energy is a polarization of orbital spin-currents that preserves the time-reversal symmetry; hence a nonmagnetic solution in accordance with experiments. The analysis brings a unifying picture of the role of exchange in the 5f shell with its relatively strong spin-orbit coupling. The results are in good accordance with recent measurements of the branching ratio for the d to f transition in the actinides.
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页数:4
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