Direct methane oxidation over Pt-modified nitrogen-doped carbons

被引：58

作者：

Soorholtz, Mario ^{[1
]}

White, Robin J. ^{[3
]}

Zimmermann, Tobias ^{[1
]}

Titirici, Maria-Magdalena ^{[3
]}

Antonietti, Markus ^{[3
]}

Palkovits, Regina ^{[1
,2
]}

Schueth, Ferdi ^{[1
]}

机构：

[1] Max Planck Inst Kohlenforsch, D-45470 Mulheim, Germany

[2] Rhein Westfal TH Aachen, D-52074 Aachen, Germany

[3] Max Planck Inst Colloids & Interfaces, D-14476 Potsdam, Germany

来源：

CHEMICAL COMMUNICATIONS | 2013年 / 49卷 / 03期

关键词：

LOW-TEMPERATURE OXIDATION; SOLID CATALYSTS; ACTIVATION; CONVERSION; CHEMICALS;

D O I：

10.1039/c2cc36232e

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Nitrogen-doped carbons derived from biomass precursors were modified with Pt2+ and successfully tested as solid catalysts in the direct oxidation of methane in fuming sulfuric acid. Remarkably, the catalytic performance was found to be substantially better than the Pt-modified Covalent Triazine Framework (CTF) system previously reported, although deactivation is more pronounced for the biomass derived catalyst supports.

引用

页码：240 / 242

页数：3

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