Catalytic Combustion of Toluene with Pd/La0.8Ce0.2MnO3 Supported on Different Zeolites

被引：16
作者：
Wang, Yongqiang [1 ,2 ]
Xiao, Li [1 ]
Zhao, Chaocheng [1 ,2 ]
Liu, Fang [1 ,2 ]
Li, Shi [1 ]
机构：
[1] China Univ Petr East China, Dept Environm & Safety Engn, Coll Chem Engn, Qingdao 266580, Peoples R China
[2] China Univ Petr East China, State Key Lab Petr Pollut Control, Dongying 257061, Peoples R China
来源：
ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY | 2018年 / 37卷 / 01期
基金：
中国国家自然科学基金;
关键词：
catalytic combustion; zeolite; perovskite; support effect; toluene; VOLATILE ORGANIC-COMPOUNDS; MANGANESE OXIDE; OXIDATION; PALLADIUM; PERFORMANCE; HYDROGEN; METHANOL; BENZENE; VOCS; PD;
D O I：
10.1002/ep.12656
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
Pd/La0.8Ce0.2MnO3 catalysts supported on various kinds of zeolites (ZSM-5, MOR, NaY, and beta) were prepared by incipient wetness impregnation method, and these catalysts were investigated by Brunauer-Emmett-Teller, X-ray diffraction analysis (XRD), Fourier transform infrared spectroscopy, and H-2-temperature programmed reduction. The catalytic activity of these catalysts was tested for toluene catalytic combustion, and the support effect was investigated. It was found that the ZSM-5 is the best support than other zeolites (MOR, NaY, and ), because it processes the higher acidity and reducibility, although its specific surface area is smaller than the others. Result of XRD indicates that Pd species are highly dispersed on the surface of the catalysts, and the doping of Pd could greatly improve the activity of La0.8Ce0.2MnO3, the light-off and complete conversion temperature of Pd/La0.8Ce0.2MnO3/ZSM-5 are only 112 and 227 degrees C, respectively. (c) 2017 American Institute of Chemical Engineers
引用
收藏
页码：215 / 220
页数：6
相关论文
共 27 条
[1]   Combustion of volatile organic compounds over supported manganese oxide:: Influence of the support, the precursor and the manganese loading [J].
Aguero, Fabiola N. ;
Scian, Alberto ;
Barbero, Bibiana P. ;
Cadus, Luis E. .
CATALYSIS TODAY, 2008, 133 :493-501
[2]   Catalytic combustion of volatile organic compounds in binary mixtures over MnOx/Al2O3 catalyst [J].
Aguero, Fabiola N. ;
Barbero, Bibiana P. ;
Gambaro, Luis ;
Cadus, Luis E. .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2009, 91 (1-2) :108-112
[3]   Supported perovskites for total oxidation of toluene [J].
Alifanti, M ;
Florea, M ;
Somacescu, S ;
Parvulescu, VI .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2005, 60 (1-2) :33-39
[4]   REVIEW - NATURAL VOLATILE ORGANIC-SUBSTANCES AND THEIR EFFECT ON AIR-QUALITY IN THE UNITED-STATES [J].
ALTSHULLER, AP .
ATMOSPHERIC ENVIRONMENT, 1983, 17 (11) :2131-2165
[5]   High pressure methane catalytic combustion over novel partially coated LaMnO3-based monoliths [J].
Barbato, Paola Sabrina ;
Di Sarli, Valeria ;
Landi, Gianluca ;
Di Benedetto, Almerinda .
CHEMICAL ENGINEERING JOURNAL, 2015, 259 :381-390
[6]   Catalytic combustion of toluene over copper oxide deposited on two types of yttria-stabilized zirconia [J].
Bialas, Anna ;
Kondratowicz, Tomasz ;
Drozdek, Marek ;
Kustrowski, Piotr .
CATALYSIS TODAY, 2015, 257 :144-149
[7]   Superior performance in catalytic combustion of toluene over mesoporous ZSM-5 zeolite supported platinum catalyst [J].
Chen, Chunyu ;
Wang, Xiong ;
Zhang, Jian ;
Bian, Chaoqun ;
Pan, Shuxiang ;
Chen, Fang ;
Meng, Xiangju ;
Zheng, Xiaoming ;
Gao, Xionghou ;
Xiao, Feng-Shou .
CATALYSIS TODAY, 2015, 258 :190-195
[8]   Enhanced performance in catalytic combustion of toluene over mesoporous Beta zeolite-supported platinum catalyst [J].
Chen, Chunyu ;
Zhu, Jie ;
Chen, Fang ;
Meng, Xiangju ;
Zheng, Xiaoming ;
Gao, Xionghou ;
Xiao, Feng-Shou .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2013, 140 :199-205
[9]   THE SORPTION OF HYDROGEN ON PALLADIUM IN A FLOW SYSTEM [J].
CHEN, G ;
CHOU, WT ;
YEH, CT .
APPLIED CATALYSIS, 1983, 8 (03) :389-397
[10]   In situ hydrothermally synthesized mesoporous LaCoO3/SBA-15 catalysts: High activity for the complete oxidation of toluene and ethyl acetate [J].
Deng, Jiguang ;
Zhang, Lei ;
Dai, Hongxing ;
Au, Chak-Tong .
APPLIED CATALYSIS A-GENERAL, 2009, 352 (1-2) :43-49
123