Non-Markovianity: initial correlations and nonlinear optical measurements

被引:17
|
作者
Dijkstra, Arend G. [1 ]
Tanimura, Yoshitaka [1 ]
机构
[1] Kyoto Univ, Dept Chem, Grad Sch Sci, Kyoto 6068502, Japan
来源
PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES | 2012年 / 370卷 / 1972期
基金
日本学术振兴会;
关键词
non-Markovianity; initial correlations; nonlinear optics; ENERGY-TRANSFER; QUANTUM; DYNAMICS; EQUATION;
D O I
10.1098/rsta.2011.0203
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
By extending the response function approach developed in nonlinear optics, we analytically derive an expression for the non-Markovianity in the time evolution of a system in contact with a quantum mechanical bath, and find a close connection with the directly observable nonlinear optical response. The result indicates that memory in the bath-induced fluctuations rather than in the dissipation causes non-Markovianity. Initial correlations between states of the system and the bath are shown to be essential for a correct understanding of the non-Markovianity. These correlations are included in our treatment through a preparation function.
引用
收藏
页码:3658 / 3671
页数:14
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