Quantum-confined stark effect in localized luminescent centers within InGaN/GaN quantum-well based light emitting diodes

被引:50
作者
De, Suman [1 ]
Layek, Arunasish [1 ]
Bhattacharya, Sukanya [1 ]
Das, Dibyendu Kumar [2 ]
Kadir, Abdul [3 ]
Bhattacharya, Arnab [3 ]
Dhar, Subhabrata [4 ]
Chowdhury, Arindam [1 ,5 ]
机构
[1] Indian Inst Technol, Dept Chem, Bombay 400076, Maharashtra, India
[2] Indian Assoc Cultivat Sci, Dept Phys Chem, Kolkata 700032, India
[3] Tata Inst Fundamental Res, Dept Condensed Matter Phys & Mat Sci, Bombay 400005, Maharashtra, India
[4] Indian Inst Technol, Dept Phys, Bombay 400076, Maharashtra, India
[5] Indian Inst Technol, Natl Ctr Photovolta Res & Educ, Bombay 400076, Maharashtra, India
关键词
MOLECULAR-BEAM EPITAXY; SPONTANEOUS POLARIZATION; EXCITON LOCALIZATION; EMISSION; DEVICES; BLUE;
D O I
10.1063/1.4754079
中图分类号
O59 [应用物理学];
学科分类号
摘要
The nature of the polarization-field in disorder induced nanoscale potential fluctuations (radiative traps) within (In,Ga)N based quantum-well (QW) heterostructures remains ambiguous. Spectrally resolved photoluminescence microscopy has been utilized to probe the local polarization field by monitoring the extent of quantum-confined Stark effect (QCSE) in radiative trap centers spontaneously formed within an (In, Ga) N QW based light emitting diode. Interestingly, two distinct categories of nanoscale radiative domains, which arise from indium compositional and interface-morphology related fluctuations of the active layers, are found to have very different degree of built-in polarization fields. Screening of QCSE in indium-rich emission centers results in blue-shift of transition energies by up to 400meV, significantly higher than that reported previously for group III-nitride based semiconductor heterostructures. A lack of correlation between the extent of QCSE and local indium mole-fractions suggests that size, shape, and strain of individual localization centers play a crucial role in modulating the local polarization field. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4754079]
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页数:5
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