Two-photon absorption of Sin (n=3-10) clusters compared with Si bulk

被引：3
作者：
Lan, You-Zhao [1 ]
机构：
[1] Zhejiang Normal Univ, Inst Phys Chem, Dept Chem, Coll Chem & Life Sci, Jinhua 321004, Zhejiang, Peoples R China
来源：
CHEMICAL PHYSICS LETTERS | 2012年 / 545卷
关键词：
NONLINEAR-OPTICAL PROPERTIES; DENSITY-FUNCTIONAL THEORY; SMALL SILICON CLUSTERS; RESPONSE FUNCTIONS; AB-INITIO; SEMICONDUCTOR CLUSTERS; CROSS-SECTIONS; POROUS SILICON; POLARIZABILITIES; NANOCLUSTERS;
D O I：
10.1016/j.cplett.2012.07.034
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The two-photon absorption (TPA) properties of the Si-n (n = 3-10) clusters were investigated by using the density functional response approach. The TPA coefficients of the Si clusters are systematically smaller than those of Si bulk for 800-2200 nm. The TPA coefficients of the Si clusters as well as Si bulk increase with a decrease of the input light wavelength. The analysis of the TPA enhancement shows that the channel of double resonance makes a significant contribution to the large TPA coefficients of the Si clusters in the visible range. (C) 2012 Elsevier B.V. All rights reserved.
引用
收藏
页码：95 / 99
页数：5
相关论文
共 50 条
[31]   Phenothiazin-N-yl-capped 1,4-diketo-3,6-diphenylpyrrolo[3,4-c]pyrrole exhibiting strong two-photon absorption and aggregation-enhanced one- and two-photon excitation red fluorescence [J].
Zhang, Kai ;
Liu, Zhongwei ;
Ying, Shian ;
Chen, Mingshuai ;
Xue, Shanfeng ;
Zhang, Haichang ;
Yang, Wenjun .
RSC ADVANCES, 2017, 7 (49) :30610-30617
[32]   The Structures of Silicon Clusters Doped with Two Gold Atoms, Si n Au2 (n=1-10) [J].
Dore, Erika M. ;
Lyon, Jonathan T. .
JOURNAL OF CLUSTER SCIENCE, 2016, 27 (04) :1365-1381
[33]   Theoretical investigation of two-photon absorption and fluorescence properties of cypridina luciferin-based derivatives: 2,3,5-trisubstituted pyrazine compounds [J].
Sun, Ying ;
Liu, Xiao-Ting ;
Guo, Jing-Fu ;
Ren, Ai-Min ;
Wang, Dan .
JOURNAL OF PHYSICAL ORGANIC CHEMISTRY, 2013, 26 (10) :822-833
[34]   Theoretical studies of one- and two-photon absorption properties for three molecules with different centers (B and N) and peripheral substituted groups [N(CH3)2 and CN] [J].
Han, De-Ming ;
Feng, Ji-Kang ;
Ren, Ai-Min ;
Shang, Xiao-Hong ;
Liu, Xiao-Juan .
JOURNAL OF LUMINESCENCE, 2009, 129 (08) :807-811
[35]   Development of a 3-body: many-body integrated fragmentation method for weakly bound clusters and application to water clusters (H2O)n=3-10, 16, 17 [J].
Bates, Desiree M. ;
Smith, Joshua R. ;
Janowski, Tomasz ;
Tschumper, Gregory S. .
JOURNAL OF CHEMICAL PHYSICS, 2011, 135 (04)
[36]   Theoretical Studies for One- and Two-photon Absorption Properties of 3,6-and 2,7-Carbazole Derivatives [J].
Li Wen-Chao ;
Feng Ji-Kang ;
Ren Ai-Min ;
Sun Chia-Chung ;
Yu Xiao-Qiang ;
Wang Jun-Jie .
CHEMICAL JOURNAL OF CHINESE UNIVERSITIES-CHINESE, 2010, 31 (01) :100-105
[37]   Efficient and Accurate Methods for the Geometry Optimization of Water Clusters: Application of Analytic Gradients for the Two-Body:Many-Body QM:QM Fragmentation Method to (H2O)n, n=3-10 [J].
Bates, Desiree M. ;
Smith, Joshua R. ;
Tschumper, Gregory S. .
JOURNAL OF CHEMICAL THEORY AND COMPUTATION, 2011, 7 (09) :2753-2760
[38]   Probing structure, thermochemistry, electron affinity, and magnetic moment of thulium-doped silicon clusters TmSin (n=3-10) and their anions with density functional theory [J].
Huang, Xintao ;
Yang, Jucai .
JOURNAL OF MOLECULAR MODELING, 2018, 24 (01)
[39]   Evolution of Vibrational Spectra in the Manganese-Silicon Clusters Mn2Sin, n=10, 12, and 13, and Cationic [Mn2Si13]+ [J].
Khanna, Vaibhav ;
Singh, Roshan ;
Claes, Pieterjan ;
Minh Tho Nguyen ;
Fielicke, Andre ;
Janssens, Ewald ;
Lievens, Peter ;
McGrady, John E. .
JOURNAL OF PHYSICAL CHEMISTRY A, 2022, 126 (10) :1617-1626
[40]   Two-photon absorption properties of star-shaped compounds based on 1,3,5-triazine and 1,3,5-trisubstituted benzene [J].
Zhou, X ;
Ren, AM ;
Feng, JK ;
Liu, XJ .
JOURNAL OF MOLECULAR STRUCTURE-THEOCHEM, 2004, 668 (2-3) :229-234
12345