Ultra-fast and ultra-intense x-ray sciences: first results from the Linac Coherent Light Source free-electron laser

被引:139
作者
Bostedt, C. [1 ]
Bozek, J. D. [1 ]
Bucksbaum, P. H. [1 ]
Coffee, R. N. [1 ]
Hastings, J. B. [1 ]
Huang, Z. [1 ]
Lee, R. W. [1 ]
Schorb, S. [1 ]
Corlett, J. N. [2 ]
Denes, P. [2 ]
Emma, P. [2 ]
Falcone, R. W. [2 ]
Schoenlein, R. W. [2 ]
Doumy, G. [3 ]
Kanter, E. P. [3 ]
Kraessig, B. [3 ]
Southworth, S. [3 ]
Young, L. [3 ]
Fang, L. [4 ]
Hoener, M. [4 ]
Berrah, N. [4 ]
Roedig, C. [5 ]
DiMauro, L. F. [5 ]
机构
[1] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA
[2] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA
[3] Argonne Natl Lab, Argonne, IL 60439 USA
[4] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA
[5] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA
基金
美国国家科学基金会;
关键词
FEMTOSECOND; SINGLE; IONIZATION; PULSES; SHELL; ATOMS; PHOTOIONIZATION; GENERATION; EXCITATION; BEAM;
D O I
10.1088/0953-4075/46/16/164003
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
X-ray free-electron lasers (FELs) produce femtosecond x-ray pulses with unprecedented intensities that are uniquely suited for studying many phenomena in atomic, molecular, and optical (AMO) physics. A compilation of the current developments at the Linac Coherent Light Source (LCLS) and future plans for the LCLS-II and Next Generation Light Source (NGLS) are outlined. The AMO instrumentation at LCLS and its performance parameters are summarized. A few selected experiments representing the rapidly developing field of ultra-fast and peak intensity x-ray AMO sciences are discussed. These examples include fundamental aspects of intense x-ray interaction with atoms, nonlinear atomic physics in the x-ray regime, double core-hole spectroscopy, quantum control experiments with FELs and ultra-fast x-ray induced dynamics in clusters. These experiments illustrate the fundamental aspects of the interaction of intense short pulses of x-rays with atoms, molecules and clusters that are probed by electron and ion spectroscopies as well as ultra-fast x-ray scattering.
引用
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页数:21
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