Systematic study of the effects of novel halogen-free anionic surface active ionic liquid on interfacial tension of water/model oil system

被引:46
作者
Zhou, Hongtao [1 ]
Zhu, Yanguang [1 ]
Peng, Tong [2 ]
Song, Yilei [1 ]
An, Jibin [1 ]
Leng, Xu [1 ]
Yi, Zewen [1 ]
Sun, Yuqian [3 ]
Jia, Han [1 ]
机构
[1] China Univ Petr East China, Coll Petr Engn, Qingdao 266580, Peoples R China
[2] PetroChina Jidong Oilfield Co, Drilling & Prod Technol Res Inst, Tangshan 063004, Peoples R China
[3] PetroChina Changqing Oilfield Co, Gas Prod Plant 1, Yinchuan 750006, Peoples R China
基金
中国国家自然科学基金;
关键词
Chemical enhanced oil recovery; Ionic liquid; Surfactant; Interfacial tension; Interaction energy; PHASE-BEHAVIOR; AGGREGATION BEHAVIOR; DODECYL-SULFATE; CRUDE-OIL; RECOVERY; IMIDAZOLIUM; CHLORIDE; TEMPERATURE; WATER;
D O I
10.1016/j.molliq.2016.08.080
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this investigation, a novel anionic-halogen-free ionic liquid (IL), 1-butyl-3-methylimidazolium dodecyl sulfate ([C(4)mim][C12SO4]), was synthesized and examined for possible application in the chemical enhanced oil recovery (EOR) processes. In this way, the effects of [C(4)mim][C12SO4] and NaCl concentrations, temperature and model oil type (aliphatic and aromatic hydrocarbons) on interfacial tensions (IFTs) between [C(4)mim][C12SO4] solutions and model oils were systematically investigated. It, is surprisingly revealed that the novel SAIL [C(4)mim][C12SO4] is highly effective in reducing the IFT of aromatic hydrocarbon/water system, and ultra-low IFT can be achieved in the presence of salinity at higher temperature. Moreover, the interaction energies between [C(4)mim][C12SO4] and different model oil molecules were calculated using molecular mechanics, which could further interpret the reasons of ultra-low IFT. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码:516 / 520
页数:5
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