The potential of enhanced weathering in the UK

被引:173
作者
Renforth, P. [1 ,2 ]
机构
[1] Univ Oxford, Dept Earth Sci, Oxford OX1 3AN, England
[2] Univ Oxford, Oxford Geoengn Programme, Oxford Martin Sch, Old Indian Inst, Oxford OX1 3BD, England
关键词
Enhanced weathering; Geoengineering; Mineral carbonation; Carbon dioxide reduction; United Kingdom; CARBON-DIOXIDE SEQUESTRATION; WHIN SILL COMPLEX; CO2; SEQUESTRATION; ATMOSPHERIC CO2; VOLCANIC GROUP; GEOCHEMISTRY; PRECIPITATION; PERIDOTITE; PETROLOGY; INTRUSION;
D O I
10.1016/j.ijggc.2012.06.011
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Enhanced weathering is the process by which carbon dioxide is sequestered from the atmosphere through the dissolution of silicate minerals on the land surface. The carbon capture potential of enhanced weathering is large, yet there are few data on the effectiveness or engineering feasibility of such a scheme. Here, an energy/carbon balance is presented together with the associated operational costs for the United Kingdom as a case study. The silicate resources are large and could theoretically capture 430 billion tonnes (Gt) of CO2. The majority of this resource is contained in basic rocks (with a carbon capture potential of similar to 0.3 tCO(2) t(-1) rock). There are a limited number of ultrabasic formations (0.8 tCO(2) t(-1) rock) with a total carbon capture potential of 25.4 GtCO(2). It is shown that the energy costs of enhanced weathering may be 656-3501 kWh tCO(2)(-1) (net CO2 draw-down, which accounts for emissions during production) for basic rocks and 224-748 kWh tCO(2)(-1) for ultrabasic rocks. Comminution and material transport are the most energy intensive processes accounting for 77-94% of the energy requirements collectively. The operational costs of enhanced weathering could be (sic)44-361 tCO(2)(-1) ($70-578 tCO(2)(-1)) and (sic)15-77 tCO(2)(-1) ($24-123 tCO(2)(-1)) for basic and ultrabasic rocks respectively. Providing sufficient weathering rates full exploitation of this resource is not possible given the environmental and amenity value of some of the rock formations. Furthermore, the weathering rate and environmental impact of silicate mineral application to the land surface is not fully understood, and further investigation in this area is required to reduce the uncertainty in the estimated costs presented here. (c) 2012 Elsevier Ltd. All rights reserved.
引用
收藏
页码:229 / 243
页数:15
相关论文
共 94 条
[1]  
[Anonymous], OR08025 BRIT GEOL SU
[2]  
[Anonymous], 2010, REV MAR TRANSP
[3]  
[Anonymous], 2009, Geoengineering the climate: Science, governance and uncertainty
[4]  
[Anonymous], 2011, GUIDELINES MEASURING
[5]  
ASAE, 1999, AGR MACH MAN DAT
[6]   Structural changes in olivine (Mg, Fe)2SiO4 mechanically activated in high-energy mills [J].
Balaz, Peter ;
Turianicova, Erika ;
Fabian, Martin ;
Kleiv, Rolf Arne ;
Briancin, Jaroslav ;
Obut, Abdullah .
INTERNATIONAL JOURNAL OF MINERAL PROCESSING, 2008, 88 (1-2) :1-6
[7]   Geochemistry of the tertiary volcanism of Northern Ireland [J].
Barrat, JA ;
Nesbitt, RW .
CHEMICAL GEOLOGY, 1996, 129 (1-2) :15-38
[8]   On the origin of a reddened interflow bed within the Palaeocene lava field of north Skye [J].
Bell, BR ;
Williamson, IT ;
Head, FE ;
Jolley, DW .
SCOTTISH JOURNAL OF GEOLOGY, 1996, 32 :117-126
[9]   GEOCARB III:: A revised model of atmospheric CO2 over phanerozoic time [J].
Berner, RA ;
Kothavala, Z .
AMERICAN JOURNAL OF SCIENCE, 2001, 301 (02) :182-204
[10]  
BGS, 1985, 73 BGS MIN REC PROGR