The Advance and Critical Functions of Energetic Carbon Dots in Carbon Dioxide Photo/Electroreduction Reactions

被引：12

作者：

Bao, Kaili ^{[1
]}

Shi, Jie ^{[1
]}

Liao, Fan ^{[1
]}

Huang, Hui ^{[1
]}

Liu, Yang ^{[1
]}

Kang, Zhenhui ^{[1
,2
]}

机构：

[1] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Jiangsu, Peoples R China

[2] Macau Univ Sci & Technol, MUST SUDA Joint Res Ctr Adv Funct Mat, Macao Inst Mat Sci & Engn MIMSE, Taipa 999078, Macao, Peoples R China

来源：

SMALL METHODS | 2022年 / 6卷 / 12期

基金：

中国国家自然科学基金; 国家重点研发计划;

关键词：

carbon dots; CO2 reduction reaction; photo/electro catalysis; PHOTOCATALYTIC CO2 REDUCTION; GRAPHENE QUANTUM DOTS; VISIBLE-LIGHT PHOTOCATALYSTS; METAL-ORGANIC FRAMEWORKS; ELECTROCHEMICAL REDUCTION; ENHANCED ACTIVITY; WATER OXIDATION; CONVERSION; HYBRID; ELECTROREDUCTION;

D O I：

10.1002/smtd.202200914

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

As a unique carbon-based nano material, carbon dots (CDs) have attracted great attention because of their special structures and properties, and have been widely used in various fields, such as bio-imaging technology, catalyst design, pollutant degradation, chemical analysis, clean energy development and so on. CDs are used as catalysts or cocatalysts for multiple energy conversion reactions due to their advantages of valid visible light utilization, fast transmission of charge carriers, excellent catalytic activity, and good electrical conductivity. This review first summarizes the basic structure and properties of CDs. The advance and critical functions of energetic CDs in carbon dioxide photo/electroreduction reactions are discussed in detail. Due to the excellent optical absorption, electron transfer properties and good conductivity of CDs, they can enhance catalytic activity and stability effectively. In the end, the existing problems and future development opportunities of CDs-based catalysts in CO2 reduction reaction are proposed and outlined.

引用

页数：19

共 50 条

[41] Bismuthene for highly efficient carbon dioxide electroreduction reaction [J].

Yang, Fa ;

Elnabawy, Ahmed O. ;

Schimmenti, Roberto ;

Song, Ping ;

Wang, Jiawei ;

Peng, Zhangquan ;

Yao, Shuang ;

Deng, Ruiping ;

Song, Shuyan ;

Lin, Yue ;

Mavrikakis, Manos ;

Xu, Weilin .

NATURE COMMUNICATIONS, 2020, 11 (01)

[42] Layered bismuth oxide/bismuth sulfide supported on carrageenan derived carbon for efficient carbon dioxide electroreduction to formate [J].

Hu, Xiangzhao ;

Sun, Junjie ;

Zheng, Wanzhen ;

Zheng, Sixing ;

Xie, Yu ;

Gao, Xiang ;

Yang, Bin ;

Li, Zhongjian ;

Lei, Lecheng ;

Hou, Yang .

CHINESE JOURNAL OF CHEMICAL ENGINEERING, 2022, 43 :116-123

[43] Kinetic Analysis on the Role of Bicarbonate in Carbon Dioxide Electroreduction at Immobilized Cobalt Phthalocyanine [J].

Zeng, Joy S. ;

Corbin, Nathan ;

Williams, Kindle ;

Manthiram, Karthish .

ACS CATALYSIS, 2020, 10 (07) :4326-4336

[44] Electrochemical impedance spectroscopy as a tool to investigate the electroreduction of carbon dioxide: A short review [J].

Sacco, Adriano .

JOURNAL OF CO2 UTILIZATION, 2018, 27 :22-31

[45] Selective Electroreduction of Carbon Dioxide over SnO2-Nanodot Catalysts [J].

Hu, Congling ;

Li, Lulu ;

Deng, Wanyu ;

Zhang, Gong ;

Zhu, Wenjin ;

Yuan, Xintong ;

Zhang, Lei ;

Zhao, Zhi-Jian ;

Gong, Jinlong .

CHEMSUSCHEM, 2020, 13 (23) :6353-6359

[46] Hierarchical micro/nanostructured silver hollow fiber boosts electroreduction of carbon dioxide [J].

Li, Shoujie ;

Chen, Wei ;

Dong, Xiao ;

Zhu, Chang ;

Chen, Aohui ;

Song, Yanfang ;

Li, Guihua ;

Wei, Wei ;

Sun, Yuhan .

NATURE COMMUNICATIONS, 2022, 13 (01)

[47] Enhanced efficiency for carbon dioxide electroreduction to formate by electrodeposition Sn on Cu nanowires [J].

Chen, Guoqian ;

Ye, Dingding ;

Chen, Rong ;

Li, Jun ;

Zhu, Xun ;

Liao, Qiang .

JOURNAL OF CO2 UTILIZATION, 2021, 44

[48] Recent progress on the electroreduction of carbon dioxide to C1 liquid products [J].

Duan, Yan-Xin ;

Cui, Rong-Chao ;

Jiang, Qing .

CURRENT OPINION IN ELECTROCHEMISTRY, 2023, 38

[49] Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel [J].

Gao, Shan ;

Lin, Yue ;

Jiao, Xingchen ;

Sun, Yongfu ;

Luo, Qiquan ;

Zhang, Wenhua ;

Li, Dianqi ;

Yang, Jinlong ;

Xie, Yi .

NATURE, 2016, 529 (7584) :68-+

[50] The electroreduction of carbon dioxide by macrocyclic cobalt complexes chemically modified on a glassy carbon electrode [J].

Aga, H ;

Aramata, A ;

Hisaeda, Y .

JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 1997, 437 (1-2) :111-118

← 1 2 3 4 5 →