Atmospheric Transport and Deposition of Mineral Dust to the Ocean: Implications for Research Needs

被引:160
|
作者
Schulz, Michael [1 ]
Prospero, Joseph M. [2 ]
Baker, Alex R. [3 ]
Dentener, Frank [4 ]
Ickes, Luisa [5 ]
Liss, Peter S. [3 ]
Mahowald, Natalie M. [6 ]
Nickovic, Slobodan [5 ]
Garcia-Pando, Carlos Perez [7 ]
Rodriguez, Sergio [8 ]
Sarin, Manmohan [9 ]
Tegen, Ina [10 ]
Duce, Robert A. [11 ,12 ]
机构
[1] Norwegian Meteorol Inst, Oslo, Norway
[2] Univ Miami, Rosenstiel Sch Marine & Atmospher Sci, Miami, FL 33149 USA
[3] Univ E Anglia, Sch Environm Sci, Norwich NR4 7TJ, Norfolk, England
[4] Commiss European Communities, JRC, Inst Environm & Sustainabil, Ispra, Italy
[5] World Meteorol Org, Geneva, Switzerland
[6] Cornell Univ, Ithaca, NY USA
[7] NASA, Goddard Inst Space Studies, New York, NY 10025 USA
[8] Izana Atmospher Res Ctr, Santa Cruz De Tenerife, Spain
[9] Phys Res Lab, Dept Planetary & Geosci, Ahmadabad 380009, Gujarat, India
[10] Leibniz Inst Tropospher Res, Leipzig, Germany
[11] Texas A&M Univ, Dept Oceanog, College Stn, TX 77843 USA
[12] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX USA
基金
美国国家科学基金会;
关键词
DRY AEOLIAN DEPOSITION; DESERT DUST; IRON SOLUBILITY; AEROSOL INTERACTIONS; PARTICLE DEPOSITION; GLOBAL DISTRIBUTION; TRACE-ELEMENTS; SAHARAN DUST; WIND EROSION; AFRICAN DUST;
D O I
10.1021/es300073u
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This paper reviews our knowledge of the measurement and modeling of mineral dust emissions to the atmosphere, its transport and deposition to the ocean, the release of iron from the dust into seawater, and the possible impact of that nutrient on marine biogeochemistry and climate. Of particular concern is our poor understanding of the mechanisms and quantities of dust deposition as well as the extent of iron solubilization from the dust once it enters the ocean. Model estimates of dust deposition in remote oceanic regions vary by more than a factor of 10. The fraction of the iron in dust that is available for use by marine phytoplankton is still highly uncertain. There is an urgent need for a long-term marine atmospheric surface measurement network, spread across all oceans. Because the southern ocean is characterized by large areas with high nitrate but low chlorophyll surface concentrations, that region is particularly sensitive to the input of dust and iron. Data from this region would be valuable, particularly at sites downwind from known dust source areas in South America, Australia, and South Africa. Coordinated field experiments involving both atmospheric and marine measurements are recommended to address the complex and interlinked processes and role of dust/Fe fertilization on marine biogeochemistry and climate.
引用
收藏
页码:10390 / 10404
页数:15
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