A time-dependent response to optical excitation in molecular junctions

被引:13
作者
Park, Tae-Ho [1 ]
Galperin, Michael [1 ]
机构
[1] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA
基金
美国国家科学基金会;
关键词
ENHANCED RAMAN-SCATTERING; SINGLE-MOLECULE; QUANTUM-INTERFERENCE; EXCITED-STATE; NONEQUILIBRIUM PROCESSES; CONJUGATED MOLECULES; CHARGE-TRANSFER; DIPOLE-MOMENT; TRANSPORT; NANOPARTICLES;
D O I
10.1088/0031-8949/2012/T151/014038
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We discuss the theoretical modeling of a time-dependent response to optical excitations in molecular junctions. The expression for a time-dependent Raman signal at non-equilibrium is proposed. The optical control of the current, Raman scattering in junctions and time-dependent correlations between charge and photon fluxes is simulated within simple models.
引用
收藏
页数:8
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共 73 条
[1]   Onset of energy dissipation in ballistic atomic wires -: art. no. 216803 [J].
Agraït, N ;
Untiedt, C ;
Rubio-Bollinger, G ;
Vieira, S .
PHYSICAL REVIEW LETTERS, 2002, 88 (21) :4
[2]   Resonant coupling between localized plasmons and anisotropic molecular coatings in ellipsoidal metal nanoparticles [J].
Ambjörnsson, T ;
Mukhopadhyay, G ;
Apell, SP ;
Käll, M .
PHYSICAL REVIEW B, 2006, 73 (08)
[3]   Strongly coupled quantum dot-metal nanoparticle systems: Exciton-induced transparency, discontinuous response, and suppression as driven quantum oscillator effects [J].
Artuso, Ryan D. ;
Bryant, Garnett W. .
PHYSICAL REVIEW B, 2010, 82 (19)
[4]   SHIFTS AND DIPS IN INELASTIC-ELECTRON-TUNNELING SPECTRA DUE TO THE TUNNEL-JUNCTION ENVIRONMENT [J].
BAYMAN, A ;
HANSMA, PK ;
KASKA, WC .
PHYSICAL REVIEW B, 1981, 24 (05) :2449-2455
[5]   Controlling quantum transport through a single molecule [J].
Cardamone, David M. ;
Stafford, Charles A. ;
Mazumdar, Sumit .
NANO LETTERS, 2006, 6 (11) :2422-2426
[6]   CDSE NANOCRYSTALS WITH A DIPOLE-MOMENT IN THE 1ST EXCITED-STATE [J].
COLVIN, VL ;
ALIVISATOS, AP .
JOURNAL OF CHEMICAL PHYSICS, 1992, 97 (01) :730-733
[7]   Charge-Transfer Enhancement Involved in the SERS of Adenine on Rh and Pd Demonstrated by Ultraviolet to Visible Laser Excitation [J].
Cui, Li ;
Wu, De-Yin ;
Wang, An ;
Ren, Bin ;
Tian, Zhong-Qun .
JOURNAL OF PHYSICAL CHEMISTRY C, 2010, 114 (39) :16588-16595
[8]   QUANTUM-THEORY OF NONEQUILIBRIUM PROCESSES .1. [J].
DANIELEWICZ, P .
ANNALS OF PHYSICS, 1984, 152 (02) :239-304
[9]   Shot noise measurements on a single molecule [J].
Djukic, D ;
van Ruitenbeek, JM .
NANO LETTERS, 2006, 6 (04) :789-793
[10]   Generation of molecular hot electroluminescence by resonant nanocavity plasmons [J].
Dong, Z. C. ;
Zhang, X. L. ;
Gao, H. Y. ;
Luo, Y. ;
Zhang, C. ;
Chen, L. G. ;
Zhang, R. ;
Tao, X. ;
Zhang, Y. ;
Yang, J. L. ;
Hou, J. G. .
NATURE PHOTONICS, 2010, 4 (01) :50-54