Experimentally determining the exchange parameters of quasi-two-dimensional Heisenberg magnets

被引:108
作者
Goddard, P. A. [1 ]
Singleton, J. [2 ]
Sengupta, P. [2 ,3 ]
McDonald, R. D. [2 ]
Lancaster, T. [1 ]
Blundell, S. J. [1 ]
Pratt, F. L. [4 ]
Cox, S. [2 ]
Harrison, N. [2 ]
Manson, J. L. [5 ]
Southerland, H. I.
Schlueter, J. A. [6 ]
机构
[1] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England
[2] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA
[3] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA
[4] Rutherford Appleton Lab, ISIS Facil, Chilton OX11 0QX, Oxfordshire, England
[5] Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA
[6] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA
关键词
D O I
10.1088/1367-2630/10/8/083025
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Though long-range magnetic order cannot occur at temperatures T > 0 in a perfect two-dimensional ( 2D) Heisenberg magnet, real quasi-2D materials will invariably possess nonzero inter-plane coupling J(perpendicular to) driving the system to order at elevated temperatures. This process can be studied using quantum Monte Carlo calculations. However, it is difficult to test the results of these calculations experimentally since for highly anisotropic materials in which the in-plane coupling is comparable with attainable magnetic fields J(perpendicular to) is necessarily very small and inaccessible directly. In addition, because of the large anisotropy, the Neel temperatures are low and difficult to determine from thermodynamic measurements. Here, we present an elegant method of assessing the calculations via two independent experimental probes: pulsed-field magnetization in fields of up to 85 T, and muon-spin rotation.
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页数:11
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