Microscopic Model for Ultrafast Remagnetization Dynamics

被引:36
作者
Chimata, Raghuveer [1 ]
Bergman, Anders [1 ]
Bergqvist, Lars [2 ]
Sanyal, Biplab [1 ]
Eriksson, Olle [1 ]
机构
[1] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden
[2] KTH Royal Inst Technol, Dept Mat Sci & Engn, Stockholm, Sweden
基金
瑞典研究理事会;
关键词
SPIN DYNAMICS; MAGNETISM; ELECTRONS;
D O I
10.1103/PhysRevLett.109.157201
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
In this Letter, we provide a microscopic model for the ultrafast remagnetization of atomic moments already quenched above the Stoner-Curie temperature by a strong laser fluence. Combining first-principles density functional theory, atomistic spin dynamics utilizing the Landau-Lifshitz-Gilbert equation, and a three-temperature model, we analyze the temporal evolution of atomic moments as well as the macroscopic magnetization of bcc Fe and hcp Co covering a broad time scale, ranging from femtoseconds to picoseconds. Our simulations show a variety of complex temporal behavior of the magnetic properties resulting from an interplay between electron, spin, and lattice subsystems, which causes an intricate time evolution of the atomic moment, where longitudinal and transversal fluctuations result in a macrospin moment that evolves highly nonmonotonically.
引用
收藏
页数:5
相关论文
共 27 条
[11]   Electron-phonon scattering dynamics in ferromagnets on ultrafast timescales: Influence of the phonon temperature [J].
Essert, Sven ;
Schneider, Hans Christian .
JOURNAL OF APPLIED PHYSICS, 2012, 111 (07)
[12]   BAND MODEL FOR MAGNETISM OF TRANSITION-METALS IN SPIN-DENSITY FUNCTIONAL FORMALISM [J].
GUNNARSSON, O .
JOURNAL OF PHYSICS F-METAL PHYSICS, 1976, 6 (04) :587-606
[13]   Theory for the dynamics of excited electrons in noble and transition metals [J].
Knorren, R ;
Bouzerar, G ;
Bennemann, KH .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2002, 14 (27) :R739-R765
[14]   Unifying ultrafast magnetization dynamics [J].
Koopmans, B ;
Ruigrok, JJM ;
Longa, FD ;
de Jonge, WJM .
PHYSICAL REVIEW LETTERS, 2005, 95 (26)
[15]  
Koopmans B, 2010, NAT MATER, V9, P259, DOI [10.1038/NMAT2593, 10.1038/nmat2593]
[16]   The ultimate view [J].
Koopmans, Bert .
NATURE MATERIALS, 2007, 6 (10) :715-716
[17]   EXCHANGE INTERACTIONS AND SPIN-WAVE STIFFNESS IN FERROMAGNETIC METALS [J].
LIECHTENSTEIN, AI ;
KATSNELSON, MI ;
GUBANOV, VA .
JOURNAL OF PHYSICS F-METAL PHYSICS, 1984, 14 (07) :L125-L128
[18]   Conditions for noncollinear instabilities of ferromagnetic materials -: art. no. 107205 [J].
Lizárraga, R ;
Nordström, L ;
Bergqvist, L ;
Bergman, A ;
Sjöstedt, E ;
Mohn, P ;
Eriksson, O .
PHYSICAL REVIEW LETTERS, 2004, 93 (10) :107205-1
[19]   Spin-lattice-electron dynamics simulations of magnetic materials [J].
Ma, Pui-Wai ;
Dudarev, S. L. ;
Woo, C. H. .
PHYSICAL REVIEW B, 2012, 85 (18)
[20]   Control of speed and efficiency of ultrafast demagnetization by direct transfer of spin angular momentum [J].
Malinowski, G. ;
Longa, F. Dalla ;
Rietjens, J. H. H. ;
Paluskar, P. V. ;
Huijink, R. ;
Swagten, H. J. M. ;
Koopmans, B. .
NATURE PHYSICS, 2008, 4 (11) :855-858