Instability scenarios for doped He-4 clusters

被引:24
|
作者
Gatica, SM [1 ]
Hernandez, ES [1 ]
Barranco, M [1 ]
机构
[1] UNIV BARCELONA,FAC FIS,DEPT ESTRUCTURA & CONSTITUENTS MAT,E-08028 BARCELONA,SPAIN
来源
JOURNAL OF CHEMICAL PHYSICS | 1997年 / 107卷 / 03期
关键词
D O I
10.1063/1.474611
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In the frame of finite range density functional (FRDF) theory, we review the systematics of energetic features of He-4(N) clusters doped with atomic or molecular impurities, as well as the instability scenario of their collective motions. It is shown that for drops up to N=500, the predictions of FRDF theory are coincident with those arising from microscopic many-body calculations that employ variational or diffusion Monte Carlo methods. For larger drops, the present description predicts a smooth approach to zero of the collective energies, a scenario that appears to support the most recent experimental data and microscopic calculations that demonstrate that the impurity is located within the bulk of the drop. (C) 1997 American Institute of Physics.
引用
收藏
页码:927 / 931
页数:5
相关论文
共 50 条
  • [11] STRUCTURE AND COLLECTIVE EXCITATIONS OF HE-4 CLUSTERS
    CHIN, SA
    KROTSCHECK, E
    PHYSICAL REVIEW B, 1992, 45 (02): : 852 - 874
  • [12] EXCITATION AND IONIZATION OF HE-4 CLUSTERS BY ELECTRONS
    BUCHENAU, H
    TOENNIES, JP
    NORTHBY, JA
    JOURNAL OF CHEMICAL PHYSICS, 1991, 95 (11): : 8134 - 8148
  • [13] TRANSFER OF HEAVY CLUSTERS IN THE REACTION C-12(HE-4,C-12)HE-4
    DEMYANOVA, AS
    ZAYATS, IY
    RUDCHIK, AT
    CHERNIEVSKII, VK
    MAKOVSKAZHETUSHKO, M
    SOVIET JOURNAL OF NUCLEAR PHYSICS-USSR, 1992, 55 (10): : 1527 - 1528
  • [14] MICROSCOPIC CALCULATION OF COLLECTIVE EXCITATIONS IN HE-4 CLUSTERS
    CHIN, SA
    KROTSCHECK, E
    PHYSICAL REVIEW LETTERS, 1990, 65 (21) : 2658 - 2661
  • [15] FRAGMENTATION CLUSTERS FORMED IN SUPERCRITICAL EXPANSIONS OF HE-4
    JIANG, T
    NORTHBY, JA
    PHYSICAL REVIEW LETTERS, 1992, 68 (17) : 2620 - 2623
  • [16] POSITRON-INDUCED CLUSTERS IN GASEOUS HE-3 AND HE-4
    FISHBEIN, M
    CANTER, KF
    BULLETIN OF THE AMERICAN PHYSICAL SOCIETY, 1977, 22 (04): : 638 - 638
  • [17] Nuclear magnetic ordering of He-3 clusters in solid He-4
    Schrenk, R
    Konig, SR
    Pobell, F
    PHYSICAL REVIEW LETTERS, 1996, 76 (16) : 2945 - 2948
  • [18] HE-4(-]P,P) HE-4 REACTION
    ARMSTRON.DD
    KEATON, PW
    LEE, YK
    KURJAN, PM
    BULLETIN OF THE AMERICAN PHYSICAL SOCIETY, 1972, 17 (01): : 153 - &
  • [19] ATOMIC IMPACT EXPERIMENTS WITH FREE HE-3 AND HE-4 CLUSTERS
    GSPANN, J
    ZEITSCHRIFT FUR PHYSIK B-CONDENSED MATTER, 1995, 98 (03): : 405 - 411